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While the ionisation laser crosses the molecular beam perpendicularly, the excitation laser intersects the crossing point at an angle of about 5° with respect to the ionisation laser. Care was taken to achieve complete overlap of the two lasers in the intersection region by using two complementary double-diaphragms at the entrance and the exit window of the detection chamber. Thus, the pump laser beam overlaps totally the packet of complexes that is to be ionised by the probe laser
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The octopus project in aimed at describing by first-principles the electron-ion dynamics in finite and extended systems under the influence of arbitrary time-dependent electromagnetic fields. The program can be freely downloaded from http//:www.tddft.org/programs/octopus. For details see M.A.L. Marques, A. Castro, G.F. Bertsch, A. Rubio, Comp. Phys. Comm. 151, 60 (2003)
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0001456831
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This technique, first introduced in K. Yabana, G.F. Bertsch, Phys. Rev. B 54, 4484 (1996) for the calculation of linear optical spectra of clusters, does not rely on perturbation theory, and is competitive with implementations in the frequency domain (A. Rubio, J.A. Alonso, X. Blase, L.C. Balbás, S.G. Louie, Phys. Rev. Lett. 77, 247 (1996); E5442 (1996))
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This technique, first introduced in K. Yabana, G.F. Bertsch, Phys. Rev. B 54, 4484 (1996) for the calculation of linear optical spectra of clusters, does not rely on perturbation theory, and is competitive with implementations in the frequency domain (A. Rubio, J.A. Alonso, X. Blase, L.C. Balbás, S.G. Louie, Phys. Rev. Lett. 77, 247 (1996); E5442 (1996))
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25544465797
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This technique, first introduced in K. Yabana, G.F. Bertsch, Phys. Rev. B 54, 4484 (1996) for the calculation of linear optical spectra of clusters, does not rely on perturbation theory, and is competitive with implementations in the frequency domain (A. Rubio, J.A. Alonso, X. Blase, L.C. Balbás, S.G. Louie, Phys. Rev. Lett. 77, 247 (1996); E5442 (1996))
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c = 2)). Inclusion of scalar relativistic effects turn out to be crucial for the proper description of the excited state properties of the Ba atom
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