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0842330704
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note
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2〉 was not determined independently by small-angle neutron scattering. Hence, we used standard scaling relations to estimate the chain dimensions
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29
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0842265865
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note
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K is varied between 1.82σ and 3.34σ. For details, see (30).
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30
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0842330642
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31
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0842287535
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note
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For semidilute and dense solutions, we only studied fully flexible chains swollen in an athermal (vacuum) solvent. Each solution consists of M = 50 chains of length N = 1000. The conformations were provided by B. Dünweg and P. Ahlrichs (32).
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33
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0842287534
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note
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For the BPA-PC model (34), we analyzed melt configurations for M = 100 chains of N = 60 chemical repeat units, which are represented by four beads each.
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39
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0842287536
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note
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pp relative to the ideal case of infinitely thin entangled lines. The present algorithm disregards intrachain entanglements. As studies on ring polymers show, they are only of minor relevance. We are currently working on a variant of the algorithm that overcomes these limitations.
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42
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0842330640
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note
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R. E. gratefully acknowledges financial support from an Emmy-Noether-Fellowship of the Deutsche Forschungsgemeinschaft and the hospitality of the Institute for Theoretical Physics at the University of California, Santa Barbara. S.K.S. is grateful to V. Lobaskin for help with some simulation data. A.S. was supported through the International Max Planck Research School for Polymer Materials Science, Mainz. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under contract DEAC04-94AL85000.
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