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Volumn 271, Issue 5256, 1996, Pages 1703-1705

Nonlinear spectroscopy on a single quantum system: Two-photon absorption of a single molecule

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EID: 0542371161     PISSN: 00368075     EISSN: None     Source Type: Journal    
DOI: 10.1126/science.271.5256.1703     Document Type: Article
Times cited : (76)

References (31)
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    • and references therein
    • For reviews, see: W M Itano, J C Bergquist, D. J Wineland, Science 237, 612 (1987), H Walther, Aust J Phys 46, 37 (1993), and references therein.
    • (1993) Aust J Phys , vol.46 , pp. 37
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  • 13
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    • g type. Two-photon excitation inhomogeneously broadened spectra of octatetraene in n-octane have been recorded [M F Granville, G R. Holtom, B E Konler. J Chem Phys 72. 467 (1980)]
    • (1973) J Chem, Phys. , vol.59 , pp. 4984
    • Hudson, B.S.1    Kohler, B.E.2
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    • 4243054898 scopus 로고
    • E. C. Lim, Ed. Academic Press, New York
    • g type. Two-photon excitation inhomogeneously broadened spectra of octatetraene in n-octane have been recorded [M F Granville, G R. Holtom, B E Konler. J Chem Phys 72. 467 (1980)]
    • (1982) Excited States , vol.6 , pp. 1
    • Schulten, K.1
  • 15
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    • g type. Two-photon excitation inhomogeneously broadened spectra of octatetraene in n-octane have been recorded [M F Granville, G R. Holtom, B E Konler. J Chem Phys 72. 467 (1980)]
    • (1980) J Chem Phys , vol.72 , pp. 467
    • Granville, M.F.1    Holtom, G.R.2    Konler, B.E.3
  • 20
    • 4243098284 scopus 로고    scopus 로고
    • note
    • The intensity of the inhomogeneous band varied by a factor of about 5 when the laser spot was moved from one place on the sample to another.
  • 22
    • 0003717424 scopus 로고
    • Plenum, New York
    • As no intensity redistribution between the zerophonon line and the phonon wing was observed, interaction with pnonons can cause only a dephasing In this case thermal heating does not change the area of the zero-phonon line [K K. Rebane, Impurity Spectra of Solids (Plenum, New York, 1970)].
    • (1970) Impurity Spectra of Solids
    • Rebane, K.K.1
  • 24
    • 0343234882 scopus 로고
    • W. P Ambrose, Th. Basché, W. E. Moerner, J Chem Phys.95, 7150 (1991); H.de Vries and D A. Wiersma, ibid 72, 1851 (1979)
    • (1979) J Chem Phys. , vol.72 , pp. 1851
    • Vries, H.D.1    Wiersma, D.A.2
  • 25
    • 4243116342 scopus 로고    scopus 로고
    • note
    • On the basis of the measurement of a few molecules only, variations of the order of about 20% were observed in the low-power linewidth, the saturation intensity, and the high-power count rate. More statistics are needed to get the real distribution of these values
  • 28
    • 0000383591 scopus 로고
    • The value is about four orders of magnitude larger than that measured at room temperature [R J. M. Anderson. G. R. Holtom, W. M. McClain, J. Chem. Phys. 70, 4310 (1979)] because of dramatic line narrowing at low temperature.
    • (1979) J. Chem. Phys. , vol.70 , pp. 4310
    • Anderson, R.J.M.1    Holtom, G.R.2    McClain, W.M.3
  • 31
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    • note
    • This work was supported by the Swiss National Science Foundation and by Eidgenossiche Technische Hochschule Zurich


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