Synthesis and characterization of Cu-TiPILCs for selective catalytic reduction of NO by propylene in the presence of oxygen and H2O: Influence of the calcination temperature, the copper content, and the cation promoter (Ce/Ag)

Industrial and Engineering Chemistry Research

Volumn 42, Issue 17, 2003, Pages 3871-3880

  Valverde, Jose L ^a   Dorado, Fernando ^a   Sánchez, Paula ^a   Asencio, Isaac ^a   Romero, Amaya ^a  

^a UNIVERSITY OF CASTILLA LA MANCHA   (Spain)

Author keywords

[No Author keywords available]

Indexed keywords

AGGLOMERATION; CALCINATION; CATALYST SELECTIVITY; CLAY; ENZYME INHIBITION; HIGH TEMPERATURE EFFECTS; ION EXCHANGE; LOW TEMPERATURE EFFECTS; NITROGEN OXIDES; OXIDATION; POROUS MATERIALS; PROPYLENE; WETTING;

COPPER LOADING;

TITANIUM COMPOUNDS;

CESIUM; COPPER COMPLEX; NITROGEN OXIDE; OXYGEN; SILVER; WATER;

CATALYSIS;

ARTICLE; CALCINATION; CATALYSIS; CHEMICAL PROCEDURES; CHEMICAL REACTION; HIGH TEMPERATURE; ION EXCHANGE; MATERIALS; POROSITY; REACTION ANALYSIS; REDUCTION; SYNTHESIS; TEMPERATURE DEPENDENCE; THERMOSTABILITY;

EID: 0041971528     PISSN: 08885885     EISSN: None     Source Type: Journal    
DOI: 10.1021/ie0209069     Document Type: Article

References (57)

1. 2 by Transient Techniques. J. Catal. 2000, 194, 250.
2. x with N-Free Reductants. Chem. Rev. 1995, 95, 209.
3. Iwamoto, M. Heterogeneous Catalysis for Removal of NO in Excess Oxygen - Progress in 1994. Catal. Today 1996, 29, 29.
4. Aylor, A. W.; Larsen, S. C.; Reimer, J. A.; Bell, A. T. An Infrared Study of NO Decomposition over Cu-ZSM-5. J. Catal. 1995, 157, 592.
5. 2. Appl. Catal. B 1995, 5, L257.
6. x. J. Catal. 1996, 158, 327.
7. 6. J. Catal. 1997, 172, 93.
8. 2 Catalysts. Part 2: Steady-State Isotopic Transient Kinetic Analysis. J. Catal, 1999, 182, 497.
9. 2 over Pd/sulfated zirconia catalysts. Catal. Today 1999, 54, 419.
10. 3. J. Catal. 1999, 184, 377.
11. Xie, S.; Rosynek, M. P.; Lunsford, J. H. Catalytic Reactions of NO over 0-7 mol % Ba/MgO Catalysts. I. The Direct Decomposition of NO. J. Catal. 1999, 188, 24.
12. Meunier, F. C.; Breen, J. P.; Zuzaniuk, V.; Olsson, M.; Ross, J. R. H. Mechanistic Aspects of the Selective Reduction of NO by Propene over Alumina and Silver-Alumina Catalysts. J. Catal. 1999, 187, 493.
13. 2 over Pd-H-Mordenite J. Catal. 2000, 195, 151.
14. Topsoe, N. Y.; Dumesic, J. A.; Topsoe, H. Vanadia-Titania Catalysts for Selective Catalytic Reduction of Nitric-Oxide by Ammonia. II. Studies of Active Sites and Formulation of Catalytic Cycles. J. Catal. 1995, 151, 241.
15. Valverde, J. L.; Sánchez, P.; Dorado, F.; Molina, C. B.; Romero, A. Influence of the Synthesis Conditions on the Preparation of Titanium Pillared Clays Using Hydrolyzed Titanium Ethoxide as the Pillaring Agent. Microporous Mesoporous Mater. 2002, 54, 155.
16. Valverde, J. L.; Canizares, P.: Sun Kou, M. R.; Molina, C. B. Enhanced Thermal Stability of Al-Pillared Smectites Modified With Ce and La. Clays Clay Miner. 2000, 48, 424.
17. Yang, R. T.; Tharappiwattananon, N.; Long, R. Q. Ion-Exchanged Pillared Clays for Selective Catalytic Reduction of NO by Ethylene in the Presence of Oxygen. Appl. Catal. B 1998, 19, 289.
18. 3 on Titanium Pillared Montmorillonite. Catal. Lett. 1996, 36, 237.
19. 2+ Ion-Exchanged Pillared Clays. Appl. Catal. B 1997, 11, 347.
20. x by Propylene. Appl. Catal. B. 2002, in press.
21. Sterte, J. Preparation and Properties of Large-Pore La-Al-Pillared Montmorillonite. Clays Clay Miner. 1991, 39, 167.
22. Booij, E.; Kloprogge, J. T.; Rob Van Veen, J. A. Preparation, Structural Characteristics and Catalytic Properties of Large-Pore Rare Earth Element (Ce, La)/Al-Pillared Smectites. Clays Clay Miner. 1996, 44, 774.
23. 2 SCR by Propene. Stud. Surf. Sci. Catal. 2002, 142, 731.
24. Valverde, J. L.; Sánchez, P.; Dorado, F.; Asencio, I.; Romero, A. Preparation and characterization of titanium pillared clays using titanium alkoxides. Influence of the synthesis parameters. Clays Clay Miner. 2002, in press.
25. Yamanaka, S.; Nishihara, T.; Hattori, M.; Suzuki, Y. Preparation and Properties of Titania Pillared Clay. Math. Chem. Phys. 1987, 17, 87.
26. Gil, A.; Diaz, A.; Montes, M.; Acosta, D. R. Characterization of the Microporosity of Pillared Clays by Nitrogen Adsorption. Application of the Horvath-Kawazoe Approach. J. Mater. Sci. 1994, 29, 4927.
27. Bahranowski, K.; Gasior, M.; Kielski, A.; Podobinski, J.; Serwicka, E. M.; Vartikian, L. A.; Wodnicka, K. Physico-Chemical Characterization and Catalytic Properties of Copper-Doped Alumina-Pillared Montmorillonites. Clays Clay Miner. 1998, 46, 98.
28. Gil, A.; Vicente, M. A.; Gandia, L. M. Main Factors Controlling the Texture of Zirconia and Alumina Pillared Clays. Microporous Mesoporous Mater. 2000, 34, 115.
29. Bahranowski, K.; Gasior, M.; Kielski, A.; Podobinski, J.; Serwicka, E. M.; Vartikian, L. A.; Wodnicka, K. Cu-doped Alumina-pillared Montmorillonites as Catalysts for Oxidation of Toluene and Xylenes with Hydrogen Peroxide. Clay Miner. 1999, 34, 79.
30. Bahranowski, K.; Dula, R.; Labanowska, M.; Serwicka, E. M. ESR Study of Cu Centers Supported on Al, Ti, and Zr-pillared Montmorillonite Clay. Appl. Spectrosc. 1996, 50, 1439.
31. Bernier, A.; Admaiai, L. F.; Grange, P. Synthesis and Characterization of Titanium Pillared Clays: Influence of the Temperature of Preparation. Appl. Catal. 1991, 72, 269.
32. Sarkany, J.; Sachtler, W. M. H. Redox chemistry of Cu/Na-ZSM-5: Detection of Cuprous Ions by FT IR. Zeolites 1994, 14, 7.
33. Bulanek, R.; Wichterlova, B.; Sobalik, Z.; Tichy, J. Reducibility and Oxidation Activity of Cu Ions in Zeolites. Effect of Cu ion Coordination and Zeolite Framework Composition. Appl. Catal. B 2001, 31, 13.
34. 2+ ESR study. J. Phys. Chem. 1995, 99, 16327.
35. Tanabe, S.; Matsumoto, H. Effect of Preliminary Treatment with Ammonia on the Reduction of CuY Zeolite. Appl. Catal. 1988, 45, 27.
36. Canizares, P.; De Lucas, A.; Dorado, F.; Duran, A.; Asencio, I. Characterization of Ni and Pd Supported on H-mordenite Catalysts: Influence of the Metal Loading Method. Appl. Catal. A 1998, 169, 137.
37. x Reduction Catalysis. Catal. Today 1997, 33, 279.
38. Chajar, Z.; Denton, P.; Berthet de Bernard, F.; Primet, M.; Praliaud, H. Influence of Silver on the Catalytic Activity of Cu-ZSM5 for NO SCR by Propane. Effect of the Presence of Water and Hydrothermal Agings. Catal. Lett. 1998, 55, 217.
39. Burch, R., Ed. Pillared Clays. Catal. Today 1987, 2, 185.
40. 2-based catalysts. Appl. Catal. B 2001, 30, 163.
41. 2O. Ind. Eng. Chem. Res. 2002, 41, 2090.
42. x Reduction with Dodecane over Cerium and Palladium Loaded Mordenite. Appl. Catal. B 2001, 33, 25.
43. Kundakovic, L. J.; Flytzani-Stephanopoulos, M. Reduction Characteristics of Copper Oxide in Cerium and Zirconium Oxide Systems. Appl. Catal. A 1998, 171, 13.
44. Li, Z.; Flytzani-Stephanopoulos, M. On the Promotion of Ag-ZSM5 by Cerium for the SCR of NO by Methane. J. Catal. 1999, 182, 313.
45. 4. Appl. Catal. B 1999, 22, 35.
46. Zhang, Y.; Flytzani-Stephanopoulos, M. Hydrothermal Stability of Cerium Modified Cu-ZSM-5 Catalyst for Nitric Oxide Decomposition. J. Catal. 1996, 164, 131.
47. Li, Z.; Leo, K.; Flytzani-Stephanopoulos, M. Selective Catalytic Reduction of Nitric Oxide by Methane over Cerium and Silver Exchanged ZSM-5 Catalysts. Fall Meeting of the Catalysis Society of New England, Worcester, MA, 1997.
48. 2+-Exchanged Pillared Clays: An IR Study of the NO Decomposition Mechanism. J. Mol. Catal A 1998, 137, 273.
49. 8. Chem. Lett. 2001, 44-45.
50. 3 ratio and cation loading. Catal. Today 2001, 68, 161-171.
51. Ma, A.-Z.; Muhler, M.; Grünert, W. Selective catalytic reduction of NO by ammonia over Raney-Ni supported Cu-ZSM-5. II. Interactions between support and supported Cu-ZSM-5. Appl. Catal. B 2000, 27, 37-47.
52. 2 in the presence of oxygen over supported silver catalysts. Appl. Catal. B 2002, 37, 205-216.
53. 2. Catal. Today 2002, 75, 373-378.
54. Asencio, I. Reducción Catalítica Selectiva de Oxidos de Nitrógeno Empleando Zeolitas Intercambiadas como Catalizador. Ph.D., University of Castilla-La Mancha, Ciudad Real, Spain, 2002.
55. x reaction. Appl. Catal. A 2001, 222, 163-181.
56. 3. J. Catal. 2000, 190, 75-91.
57. Fliatoura, K. D.; Verykios, X. E.; Costa, C. N.; Efstathiou, A. M. Selective catalytic reduction of nitric oxide by methane in the presence of oxygen over CaO catalyst. J. Catal. 1999, 183, 323-335.