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Volumn 102, Issue 45, 1998, Pages 9081-9090

Singlet-state electron transfer between a porphyrin and ubiquinone: A transient resonance raman and quantum chemical study

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EID: 0041920765     PISSN: 10895647     EISSN: None     Source Type: Journal    
DOI: None     Document Type: Article
Times cited : (5)

References (95)
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    • Academic Press: New York, and references therein
    • (a) For extensive literature on related bimolecular ET processes, see: Kalyanasundaram, K. Photochemistry of Polypyridine and Porphyrin Complexes; Academic Press: New York, 1992; pp 450-478 and references therein. (b) Hug, G. L.; Marciniak, B.; J. Phys. Chem. 1995, 99, 1478 and references therein. (c) Logunov, S. L.; Rodgers, M. A. J. J. Photochem. Photobio. A 1997, 105, 55-63.
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    • and references therein
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    • note
    • 0 complexed pair are assumed to be stacked in a face-to-face configuration; thus, the π orbital interaction mediates ET quenching
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    • Recently other methods depending on the analysis of resonance Raman profiles of charge-transfer absorption bands as way of obtaining reorganization energies have been published, e.g.: (a) Markel, F.; Ferris, N. S.; Gould, I. R.; Myers, A. B. J. Chem. Soc. 1992, 114, 6208. (b) Kulinowski, K.; Gould, I. R.; Myers, A. B. J. Phys. Chem. 1995, 99, 9017. (c) Doorn S. K.; Hupp, J. T. J. Am. Chem. Soc. 1989, 111, 1142.
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    • Recently other methods depending on the analysis of resonance Raman profiles of charge-transfer absorption bands as way of obtaining reorganization energies have been published, e.g.: (a) Markel, F.; Ferris, N. S.; Gould, I. R.; Myers, A. B. J. Chem. Soc. 1992, 114, 6208. (b) Kulinowski, K.; Gould, I. R.; Myers, A. B. J. Phys. Chem. 1995, 99, 9017. (c) Doorn S. K.; Hupp, J. T. J. Am. Chem. Soc. 1989, 111, 1142.
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    • Recently other methods depending on the analysis of resonance Raman profiles of charge-transfer absorption bands as way of obtaining reorganization energies have been published, e.g.: (a) Markel, F.; Ferris, N. S.; Gould, I. R.; Myers, A. B. J. Chem. Soc. 1992, 114, 6208. (b) Kulinowski, K.; Gould, I. R.; Myers, A. B. J. Phys. Chem. 1995, 99, 9017. (c) Doorn S. K.; Hupp, J. T. J. Am. Chem. Soc. 1989, 111, 1142.
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    • note
    • (c) Unpublished data of Wheeler et al. gives an upper estimate of the reorganization energy of ubiquinone-1 of ≈0.69 eV using hybrid Hartree-Fock/density-functional approaches with large basis sets.
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    • note
    • s.
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    • -1 limit have been reported e.g.: Åkesson, E.; Walker, G. C.; Barbara, P. F. J. Chem. Phys. 1991, 91, 4188 Åkesson, E.; Johnson, A. E.; Levinger, N. E.; Walker, G. C.; DuBruil, T. B.; Barbara, P. F. J. Chem. Phys. 1992, 96, 7859. In the case of the inverted region from multiple vibrational states, and thus the BET rate is weakly dependent obtains for activationless processes; for a good discussion, see: Bixon, M.; Jortner, J. Chem. Phys. 1993, 176, 467.
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    • -1 limit have been reported e.g.: Åkesson, E.; Walker, G. C.; Barbara, P. F. J. Chem. Phys. 1991, 91, 4188 Åkesson, E.; Johnson, A. E.; Levinger, N. E.; Walker, G. C.; DuBruil, T. B.; Barbara, P. F. J. Chem. Phys. 1992, 96, 7859. In the case of the inverted region from multiple vibrational states, and thus the BET rate is weakly dependent obtains for activationless processes; for a good discussion, see: Bixon, M.; Jortner, J. Chem. Phys. 1993, 176, 467.
    • (1992) J. Chem. Phys. , vol.96 , pp. 7859
    • Åkesson, E.1    Johnson, A.E.2    Levinger, N.E.3    Walker, G.C.4    DuBruil, T.B.5    Barbara, P.F.6
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    • -1 limit have been reported e.g.: Åkesson, E.; Walker, G. C.; Barbara, P. F. J. Chem. Phys. 1991, 91, 4188 Åkesson, E.; Johnson, A. E.; Levinger, N. E.; Walker, G. C.; DuBruil, T. B.; Barbara, P. F. J. Chem. Phys. 1992, 96, 7859. In the case of the inverted region from multiple vibrational states, and thus the BET rate is weakly dependent obtains for activationless processes; for a good discussion, see: Bixon, M.; Jortner, J. Chem. Phys. 1993, 176, 467.
    • (1993) Chem. Phys. , vol.176 , pp. 467
    • Bixon, M.1    Jortner, J.2
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    • and references therein
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    • note
    • 43


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