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Volumn 8, Issue 10, 1996, Pages 2468-2480

Conversion of [(tBuCH2)2TaN]5 to Cubic TaN: Related Syntheses, EHMO Calculations, and MAS and Spin Echo 15N NMR Spectroscopies

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EID: 0037617398     PISSN: 08974756     EISSN: None     Source Type: Journal    
DOI: 10.1021/cm960034z     Document Type: Article
Times cited : (24)

References (91)
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    • For related CVD of groups 4 and 5 nitrides via chemically similar ammonolyses, see: (a) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Chem. Mater. 1993, 5, 614-619. (b) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Chem. Mater. 1991, 3, 1138-1148. (c) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Chem. Mater. 1990, 2, 235-241. (d) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. J. Am. Chem. Soc. 1990, 112, 7833-7835. (e) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Mater. Res. Soc. Proc. 1990, 168, 357-362.
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    • For related CVD of groups 4 and 5 nitrides via chemically similar ammonolyses, see: (a) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Chem. Mater. 1993, 5, 614-619. (b) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Chem. Mater. 1991, 3, 1138-1148. (c) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Chem. Mater. 1990, 2, 235-241. (d) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. J. Am. Chem. Soc. 1990, 112, 7833-7835. (e) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Mater. Res. Soc. Proc. 1990, 168, 357-362.
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    • For related CVD of groups 4 and 5 nitrides via chemically similar ammonolyses, see: (a) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Chem. Mater. 1993, 5, 614-619. (b) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Chem. Mater. 1991, 3, 1138-1148. (c) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Chem. Mater. 1990, 2, 235-241. (d) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. J. Am. Chem. Soc. 1990, 112, 7833-7835. (e) Fix, R. M.; Gordon, R. G.; Hoffman, D. M. Mater. Res. Soc. Proc. 1990, 168, 357-362.
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    • For general references on the structure of tantalum nitrides, see: (a) Terao, N. Jpn. J. Appl. Phys. 1971, 10, 248-259. (b) Schönberg, N. Acta Chem. Scand. 1954, 8, 199-203.
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    • For information regarding cubic TaN and related carbides, see: (a) Gatterer, J.; Dufek, G.; Ettmayer, P.; Kieffer, R. Monatsh. Chem. 1975, 706, 1137-1147. (b) Petrunin, V. F.; Sorokin, N. I. Izv. Akad. Nauk SSR, Neorg. Mater. 1982, 18, 2005-2008. (c) Boiko, L. G.; Popova, S. V. JETP Lett. 1970, 12, 70-71. (d) Kieffer, R.; Ettmayer, P.; Freundhofmeier, M.; Gatterer, J. Monatsh. Chem. 1971, 102, 483-485. (e) Matsumoto, O.; Konuma, M.; Kanzaki, Y. J. Less-Common Met. 1978, 60, 147-149.
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    • Gatterer, J.1    Dufek, G.2    Ettmayer, P.3    Kieffer, R.4
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    • For information regarding cubic TaN and related carbides, see: (a) Gatterer, J.; Dufek, G.; Ettmayer, P.; Kieffer, R. Monatsh. Chem. 1975, 706, 1137-1147. (b) Petrunin, V. F.; Sorokin, N. I. Izv. Akad. Nauk SSR, Neorg. Mater. 1982, 18, 2005-2008. (c) Boiko, L. G.; Popova, S. V. JETP Lett. 1970, 12, 70-71. (d) Kieffer, R.; Ettmayer, P.; Freundhofmeier, M.; Gatterer, J. Monatsh. Chem. 1971, 102, 483-485. (e) Matsumoto, O.; Konuma, M.; Kanzaki, Y. J. Less-Common Met. 1978, 60, 147-149.
    • (1982) Izv. Akad. Nauk SSR, Neorg. Mater. , vol.18 , pp. 2005-2008
    • Petrunin, V.F.1    Sorokin, N.I.2
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    • For information regarding cubic TaN and related carbides, see: (a) Gatterer, J.; Dufek, G.; Ettmayer, P.; Kieffer, R. Monatsh. Chem. 1975, 706, 1137-1147. (b) Petrunin, V. F.; Sorokin, N. I. Izv. Akad. Nauk SSR, Neorg. Mater. 1982, 18, 2005-2008. (c) Boiko, L. G.; Popova, S. V. JETP Lett. 1970, 12, 70-71. (d) Kieffer, R.; Ettmayer, P.; Freundhofmeier, M.; Gatterer, J. Monatsh. Chem. 1971, 102, 483-485. (e) Matsumoto, O.; Konuma, M.; Kanzaki, Y. J. Less-Common Met. 1978, 60, 147-149.
    • (1970) JETP Lett. , vol.12 , pp. 70-71
    • Boiko, L.G.1    Popova, S.V.2
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    • Kieffer, R.1    Ettmayer, P.2    Freundhofmeier, M.3    Gatterer, J.4
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    • For information regarding cubic TaN and related carbides, see: (a) Gatterer, J.; Dufek, G.; Ettmayer, P.; Kieffer, R. Monatsh. Chem. 1975, 706, 1137-1147. (b) Petrunin, V. F.; Sorokin, N. I. Izv. Akad. Nauk SSR, Neorg. Mater. 1982, 18, 2005-2008. (c) Boiko, L. G.; Popova, S. V. JETP Lett. 1970, 12, 70-71. (d) Kieffer, R.; Ettmayer, P.; Freundhofmeier, M.; Gatterer, J. Monatsh. Chem. 1971, 102, 483-485. (e) Matsumoto, O.; Konuma, M.; Kanzaki, Y. J. Less-Common Met. 1978, 60, 147-149.
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    • note
    • Combustion analyses of 3 may not be wholly accurate due to the stability of the nitrides and carbides of tantalum. For TaN (5), the modified Kjeldahl analysis was used because commercial combustion analyses proved to be irreproducible. On the basis of the modified Kjeldahl analysis, assuming all "vacancies" are filled with carbon, the maximum possible %C is 1.23.
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    • 0.8 (5) quite plausibly occurs on the time scale of annealing (72 h) at 800 °C but is far less likely to occur during the formation (24 h, 400 °C) of amorphous TaN (4). See: Kingery, W. D.; Bowen, H. K.; Ulmann, D. R. Introduction to Ceramics, 2nd ed.; John Wiley & Sons: New York, 1976.
    • (1976) Introduction to Ceramics, 2nd Ed.
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