Wave-packet-assisted decomposition of femtosecond transient ultraviolet-visible absorption spectra: Application to excited-state intramolecular proton transfer in solution

Journal of Physical Chemistry A

Volumn 105, Issue 14, 2001, Pages 3443-3453

  Ernsting, N P ^a   Kovalenko, S A ^a   Senyushkina, T ^a   Saam, J ^a   Farztdinov, V ^a  

^a HUMBOLDT UNIVERSITY   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

WAVE-PACKET ASSISTED DECOMPOSITION;

ABSORPTION SPECTROSCOPY; CHARGE TRANSFER; DECOMPOSITION; FREQUENCY MODULATION; GROUND STATE; MOLECULES; OPTICAL PUMPING; OSCILLATIONS; ULTRAVIOLET SPECTROSCOPY;

MOLECULAR VIBRATIONS;

EID: 0035849245     PISSN: 10895639     EISSN: None     Source Type: Journal    
DOI: 10.1021/jp003298o     Document Type: Article

References (53)

1. Mukamel, S. Principles of Nonlinear Optical Spectroscopy, Oxford University Press: New York, 1994; Chapter 10 ff.
2. Chesnoy, J.; Mokhtari, A. Phys. Rev. A 1988, 38, 3566.
3. Yang, T.-S.; Chang, M.-S.; Chang, R.; Hayashi, M.; Lin, S. H.; Vöhringer, P.; Dietz, W.; Scherer, N. F. J. Chem. Phys. 1999, 110, 12070.
4. Brito Cruz, C. H.; Fork, R. L.; Knox, W. H.; Shank, C. V. Chem. Phys. Lett. 1986, 132, 341.
5. Lenderink, E.; Duppen, K.; Wiersma, D. J. Phys. Chem. 1995, 99, 8972.
6. Thomsen, C. L.; Thogersen, J.; Keiding, S. R. J. Phys. Chem. A 1998, 102, 1062.
7. Yamaguchi, S.; Hamaguchi, H.; J. Chem. Phys. 1998, 109, 1397.
8. Alfano, R. R.; Shapiro, S. L. Phys. Rev. Lett. 1970, 24, 584.
9. Shank, C. V.; Yen, R.; Fork, L.; Orenstein, J.; Baker, G. L. Phys. Rev. Lett. 1982, 49, 1660.
10. Fork, R. L.; Shank, C. V.; Hirliman, C.; Yen, R.; Tomlinson, W. J. Opt. Lett. 1983, 8, 1.
11. Kang, T. J.; Yu, J.; Berg, M. J. Chem. Phys. 1991, 94, 2413.
12. Murakami, H.; Kinoshita, S.; Hirata, Y.; Okada, T.; Mataga, N. J. Chem. Phys 1992, 97, 7881.
13. Nishiyama, K.; Asano, Y.; Nashimoto, N.; Okada, T. J. Mol. Liq. 1995, 65/66, 41.
14. Eilers-König, N.; Kühne, T.; Schwarzer, D.; Vöringer, P.; Schroeder, J. Chem. Phys. Lett. 1996, 253, 69.
15. Müller, M. G.; Hucke, M.; Reus, M.; Holzwarth, A. R. J. Phys. Chem. 1996, 100, 9527.
16. Ruthmann, J.; Kovalenko, S. A.; Ernsting, N. P.; Ouw D. J. Chem. Phys. 1998, 109, 5466.
17. Kovalenko, S. A.; Schanz, R.; Farztdinov, V. M.; Hennig, H.; Ernsting, N. P. Chem. Phys. Lett. 2000, 323, 312.
18. Kovalenko, S. A.; Dobryakov, A. L.; Ruthmann, J.; Ernsting, N. P. Phys. Rev. A 1999, 59, 2369.
19. Seel, M.; Engleitner, S.; Zinth, W. Chem. Phys. Lett. 1997, 275, 363.
20. Arnaut, L. G.; Formosinho S. J. J. Photochem. Photobiol A: Chem. 1993, 75, 21.
21. Ormson, S. M.; Brown, R. G. Prog. React. Kinet. 1994, 19, 45.
22. Douhal, A.; Lahmani, F.; Zewail, A. H. Chem. Phys. 1996, 207, 477.
23. Perrin, C. L.; Nielson, J. B. Annu. Rev. Phys. Chem. 1997, 48, 511.
24. Chudoba, C.; Riedle, E.; Pfeiffer, M.; Elsaesser, T. Chem. Phys. Lett. 1996, 263, 622.
25. Lochbrunner, S.; Wurzer, A. J.; Riedle, E. J. Chem. Phys. 2000, 112, 10699.
26. Arthen-Engeland, Th.; Bultmann, T.; Ernsting, N. P.; Rodriguez, M. A.; Thiel, W. Chem. Phys. 1992, 163, 43.
27. Douhal, A.; Lahmani, F.; Zehnacker-Rentien, A.; Amat-Guerri, F. J. Phys. Chem. 1994, 98, 12198.
28. Pfeiffer, M.; Lenz, K.; Lau, A.; Elsaesser, T. J. Roman Spectrosc. 1995, 26, 607.
29. Pfeiffer, M.; Lenz, K.; Lau, A.; Elsaesser, T.; Steinke, T. J. Roman Spectrosc. 1997, 28, 61.
30. Ernsting, N. P. J. Phys. Chem. 1985, 89, 4932.
31. Ernsting, N. P.; Arthen-Engeland, Th.; Rodriguez, M. A.; Thiel, W. J. Chem. Phys. 1992, 97, 3914.
32. Vdovin, A.; Sepiol, J.; Jasny, J.; Kauffman, J. M.; Mordzinski, A. Chem. Phys. Lett. 1998, 296, 557.
33. Pfeiffer, M.; Lau., A.; Lenz, K.; Elsaesser, T. J. Phys. Chem. 1997, 268, 258.
34. Sobolewski, A. L.; Domcke, W. Chem. Phys. 1994, 184, 115.
35. Sobolewski, A. L.; Domcke, W. Chem. Phys. 1998, 232, 257.
36. Sobolewski, A. L.; Domcke, W. J. Phys. Chem. A 1999, 103, 4494.
37. Orlando jun., C. M.; Wirth, J. G:; Heath, D. R. Chem. Commun. 1971, 1551.
38. Mordzinski, A.; Grabowska, A.; Kühnle, W.; Krowczyn, A. Chem. Phys. Lett. 1983, 101, 291.
39. Brackmann, U.; Ernsting, N. P.; Ouw, D.; Schmitt, K. Chem. Phys. Lett. 1984, 110, 319.
40. Mordzinski, A.; Grabowska, A.; Teuchner, K. Chem. Phys. Lett. 1984, 111, 383.
41. Mordzinski, A.; Kühnle, W. J. Phys. Chem. 1986, 90, 1455.
42. Dick, B. Ber. Bunsen-Ges. Phys. Chem. 1987, 91, 1205.
43. Grabowska, A.; Mordzinski, A.; Tamai, N.; Yoshihara, K. Chem. Phys. Lett. 1988, 153, 389.
44. Grabowska, A.; Mordzinski, A.; Kownacki, K.; Gilabert, E.; Rullière, C. Chem. Phys. Lett. 1991, 177, 17.
45. Grabowska, A.; Sepiol, J.; Rullière, C. J. Phys. Chem. 1991, 95, 10493.
46. Mühlpfordt, A.; Even, U.; Ernsting, N. P. Chem. Phys. Lett. 1996, 263, 178.
47. Wortmann, R.; Lebus, S.; Reis, H.; Grabowska, A.; Kownacki, K.; Jarosz, S. Chem. Phys. 1999, 243, 295.
48. Press, W. H.; Teukolsky, S. A.; Vetterling, W. T.; Flannery, B. P. Numerical Recipes in Fortran, 2nd ed.; Cambridge Univerity Press: New York, 1992.
49. Chen, W.-G.; Braiman, M. S. J. Photochem. Photobiol. 1991, 54, 905.
50. 3 ± 7 for the range λ = 350-670 nm and 76 fs is the average. Spectral change beyond 670 nm is small and does not influence the analysis which is therefore extended to 714 nm.
51. The number of species may be larger than the number of independent basis functions (see ref 49).
52. th, proportional to the last (fourth) column of Q by construction.
53. Stewart, J. J. P. J. Comput. Chem. 1989, 10, 209.