Raman free-induction-decay measurements in low viscosity and supercooled toluene: vibrational dephasing by shear fluctuations

Journal of Chemical Physics

Volumn 114, Issue 8, 2001, Pages 3662-3673

  Hubble, Hugh W ^a   Lai, Tianshu ^a   Berg, Mark A ^a  

^a UNIVERSITY OF SOUTH CAROLINA   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

COMPUTER SIMULATION; DYE LASERS; LASER PULSES; MATHEMATICAL MODELS; MOLECULAR STRUCTURE; MOLECULAR VIBRATIONS; NEODYMIUM LASERS; NUMERICAL ANALYSIS; RAMAN SCATTERING; THERMAL EFFECTS; TOLUENE; VISCOSITY OF LIQUIDS;

COLLISIONAL DYNAMICS; DIFFUSIVE DYNAMICS; KUBO MODEL; LOW VISCOSITY TOLUENE; RAMAN FREE INDUCTION DECAY MEASUREMENT; SHEAR FLUCTUATION; SUPERCOOLED TOLUENE; VIBRATIONAL DEPHASING; VISCOELASTIC THEORY OF DEPHASING;

MOLECULAR DYNAMICS;

EID: 0035248818     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.1343872     Document Type: Article

References (58)

1. D. W. Oxtoby, Adv Chem. Phys. 40, 1 (1979).
2. A. Morresi, L. Mariani, M. R. Distefano, and M G. Giorgini, J. Raman Spectrosc. 26, 179 (1995).
3. M. D. Fayer, Ultrafast Infrared and Raman Spectroscopy (Dekker, New York, 2001).
4. D. McMorrow, W. T. Lotshaw, and G. A. Kenney-Wallace, IEEE J. Quantum Electron. 24, 443 (1988).
5. S. J. Rosenthal, X. L. Xie, M. Du, and G. R. Fleming, J Chem Phys. 95, 4715 (1991).
6. R. Jimenez, G. R. Fleming, P. V. Kumar, and M. Maroncelli, Nature (London) 369, 471 (1994).
7. M. L. Horng, J. A. Gardecki, A. Papazyan, and M. Maroncelli, J. Phys. Chem. 99, 17311 (1995).
8. D. S. Larsen, K. Ohta, and G. R. Fleming, J. Chem. Phys. 111, 8970 (1999).
9. M. Berg, Chem. Phys. Lett 228, 317 (1994).
10. J. Ma, D. A. Vanden Bout, and M. Berg, J. Chem. Phys. 103, 9146 (1995).
11. J. Ma, J. T. Fourkas, D. A. Vanden Bout, and M. Berg, in Supercooled Liquids: Advances and Novel Applications, edited by J. T. Fourkas, D. Kivelson, U. Mohanty, and K. A. Nelson (American Chemical Society, Washington, DC, 1997), Vol. 676, p. 199.
12. M. Berg, J. Phys. Chem. A 102, 17 (1998).
13. M. A. Berg, J. Chem. Phys. 110, 8577 (1999).
14. 2 to give Δ in frequent units.
15. S. F. Fischer and A. Laubereau, Chem. Phys Lett. 35, 6 (1975).
16. D. W. Oxtoby, J. Phys. Chem. 70, 2605 (1979).
17. H. Menu, D. W. Oxtoby, and K. F. Freed, Phys. Rev. A 15, 361 (1977).
18. R. M. Lynden-Bell, Mol. Phys. 33, 907 (1977).
19. R. K. Wertheimer, Mol. Phys. 35, 257 (1978).
20. R Ouillon, V. Sergiescu, and R. Tascón D'León, Mol. Phys. 49, 151 (1983).
21. T Fukuda, S. Ikawa, and M. Kimura, Chem. Phys. 133, 137 (1989).
22. J. Schroeder, V. H. Schiemann, P T. Sharko, and J. Jonas, J. Chem. Phys. 66, 3215 (1977).
23. K. S. Schweizer and D. Chandler, J. Chem. Phys. 76, 2296 (1982).
24. S. M. George and C. B. Harris, J. Chem. Phys. 77, 4781 (1982).
25. L. J. Muller, D. A. Vanden Bout, and M. Berg, J. Chem. Phys. 99, 810 (1993).
26. D. Vanden Bout, L. J. Muller, and M. Berg, Phys. Rev. Lett. 67, 3700 (1991).
27. A. Tokmakoff and M. D. Fayer, J. Chem. Phys. 103, 2810 (1995).
28. A. Tokmakoff, D. Zimdars, R. S. Urdahl, R. S. Francis, A. S. Kwok, and M. D. Fayer, J. Phys. Chem. 99, 13310 (1995).
29. K. D. Rector, M. A. Berg, and M. D. Fayer, J. Phys. Chem. B (in press).
30. A M Levine, M. Shapiro, and E. Pollak, J. Chem. Phys. 88, 1959 (1988).
31. D W Oxtoby and S. A. Rice, Chem. Phys. Lett. 42, 1 (1976).
32. D I Diestler, Chem. Phys. Lett. 39, 39 (1976).
33. D S Knauss, Mol. Phys. 36, 413 (1978).
34. D Sanitos and T. Dorfmüller, Chem. Phys. Lett. 117, 165 (1985).
35. I Ishibashi and H. Hamaguchi, J. Chem. Phys. 103, 1 (1995).
36. B. J. Berne and G. D. Harp, Adv. Chem. Phys. 17, 63 (1970).
37. J P. Boon and S. Yip, Molecular Hydrodynamics (Dover, New York, 1980).
38. R. Zwanzig and R. D. Mountain, J. Chem. Phys. 43, 4464 (1965).
39. P. W. Anderson, J. Phys. Soc. Jpn. 9, 316 (1954).
40. R. Kubo, in Fluctuation, Relaxation and Resonance in Magnetic Systems, edited by D. Ter Haar (Oliver and Boyd, London, 1961), p. 23.
41. D. Vanden Bout and M. Berg, J. Raman Spectrosc. 26, 503 (1995).
42. C. Alba, L. E. Busse, D. J. List, and C. A. Angell, J. Chem. Phys. 92, 617 (1990).
43. O. Yamamuro, I. Tsukushi, A. Lindqvist, S. Takahara, M. Ishikawa, and T. Matsuo, J. Phys. Chem. B 102, 1605 (1998).
44. J. K. Wilmshurst and H. J. Bernstein, Can. J. Chem. 35, 911 (1957).
45. C. La Lau and R. G. Snyder, Spectrochim. Acta, Part A 27, 2073 (1971).
46. N. Fuson, C. Garrigou-Lagrange, and M. L. Josien, Spectrochim. Acta 16, 106 (1960).
47. W. J. Balfour and Y. Fried, Can. J. Phys. 72, 1218 (1994).
48. A. J. Barlow, J. Lamb, and A. J. Matheson, Proc. R. Soc. London, Ser. A 292, 322 (1966).
49. CRC Handbook of Thermophysical and Thermochemical Data, edited by D. R. Lide and H. V. Kehiaian (CRC Press, Boca Raton, 1994).
50. A. Kummrow, A. Lau, and H. G. Ludewig, Opt. Commun. 107, 137 (1994).
51. T. Lai and M. A. Berg (unpublished).
52. W. G. Rothschild, M. Perrot, and J Lascombe, Chem. Phys. Lett. 78, 197 (1981).
53. M. A. Berg, in Ref. 3.
54. R. Chelli, G. Cardini, P. Procacci, R. Righini, S. Califano, and A. Albrecht, J. Chem. Phys. 113, 6851 (2000).
55. C. Levy and G. D'Arrigo, Mol. Phys. 50, 917 (1983).
56. D. van der Putten, G. Diezemann, F. Fujara, K. Hartmann, and H. Sillescu, J. Chem. Phys. 96, 1748 (1992).
57. D. R. Bauer, G. R. Alms, J. I. Brauman, and R. Pecora, J. Chem. Phys. 61, 2255 (1974).
58. M. Berg and D. A. Vanden Bout, Acc. Chem. Res. 30, 65 (1997).