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Here we restrict the word dimensionality to coordination bonds, a two dimensional system is one where coordination bonds (metal - cyanides, for example) spread in the two directions of space.
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85152990557
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note
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III.
-
-
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41
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85153017597
-
-
note
-
MT has no real meaning because at this temperature the magnetization is field dependent, nevertheless the high value indicates the presence of a large correlation within the layers.
-
-
-
-
42
-
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85152998986
-
-
note
-
It was checked that ac susceptibility vs. temperature plots performed at 0 and 50 Oe static applied field are identical to those of Figure 6 which indicate that saturation effects are nonexistent at such low fields. On the other hand, such measurements made at different frequencies of the oscillating field and with zero static field confirm the presence of a magnetic ordering at T = 14 K.
-
-
-
-
44
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85153000650
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note
-
We must be cautious at this stage because our measurements were carried out on a powder and not on an oriented single crystal with the applied field parallel to the easy axis, but the shape of the M = f(H) curve, which is the sum of the parallel and the perpendicular components of the magnetization, presents a too sharp transition to be that of a spin-flop phase.
-
-
-
-
46
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85153012657
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note
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For the previously reported cyclam-based compound, the largest susceptibility value measured (within the same applied field as for the present compound i.e. 30 Oe) was found to be one order of magnitude smaller than for the present compound.
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