The ultrafast optical Kerr effect in liquid fluoroform: An estimate of the collision-induced contribution

Physical Chemistry Chemical Physics

Volumn 2, Issue 12, 2000, Pages 2691-2697

  Laurent, Thomas F ^a   Hennig, Horst ^a   Ernsting, Nikolaus P ^a   Kovalenko, Sergey A ^a  

^a HUMBOLDT UNIVERSITY   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

FLUOROFORM;

ANISOTROPY; ARTICLE; CHEMICAL REACTION; MOLECULAR DYNAMICS; OPTICAL ROTATION; REACTION ANALYSIS;

EID: 0034659371     PISSN: 14639076     EISSN: None     Source Type: Journal    
DOI: 10.1039/b000914h     Document Type: Article

References (55)

1. 1 P. Madden and D. Kivelson, Adv. Chem. Phys., 1984, 56, 467.
2. 2 D. Frenkel and J. P. McTague, J. Chem. Phys., 1980, 72, 2801.
3. 3 A. Borysov and L. Frommhold, Adv. Chem. Phys., 1989, 75, 439.
4. 4 W. A. Steele, Adv. Chem. Phys., 1976, 34, 1.
5. 5 A. Gerschel, I. Dimicoli, J. Jaffre and A. Riou, J. Mol. Phys., 1976, 32, 679.
6. 6 A. Gerschel, C. Brot, I. Dimicoli and A. Riou, J. Mol. Phys., 1977, 33, 527.
7. 7 A. Gerschel, J. Mol. Liq., 1983, 25, 51.
8. 8 A. Gerschel, J. Mol. Phys., 1976, 31, 209.
9. 9 G. Glockler and W. F. Edgell, J. Chem. Phys., 1941, 9, 224.
10. 10 R. W. Kirk and P. W. Wilt, J. Mol. Spectrosc., 1975, 58, 102.
11. 11 J. DeZwaan, D. Hess and C. S. Johnson, Jr., J. Chem. Phys., 1975, 63, 422.
12. 12 E. W. Lang, F. X. Prielmeier, H. Radkowitsch and H.-D. Lüdemann, J. Phys. Chem., 1987, 91, 1025.
13. 13 K. L. Ramaswamy, Proc. Indian. Acad. Sci., Sect. A, 1935, 2, 360.
14. 14 H. Sutter and R. H. Cole, J. Chem. Phys., 1970, 52, 132.
15. 15 C. K. Miller, B. J. Orr and J. F. Ward, J. Chem. Phys., 1981, 74, 4858.
16. 16 S. P. Karna and M. Dupuis, Chem. Phys. Lett., 1990, 171, 201.
17. 17 R. Kobayashi, R. D. Amos, H. Koch and P. Jørgensen, Chem. Phys. Lett., 1996, 253, 374.
18. 18 K. Reuter, S. Rosenzweig and E. U. Franck, Physica A, 1989, 156, 294.
19. 19 D. Bertolini, M. Cassettari and G. Salvetti, J. Mol. Liq., 1984, 28, 175.
20. 20 P. Graf and A. Nitzan, Chem. Phys., 1998, 235, 297.
21. 21 H. J. Böhm, R. Ahlrichs, P. Scharf and H. Schiffer, J. Chem. Phys., 1984, 81, 1389.
22. 22 Y. C. Hou and J. J. Martin, AIChE J., 1957, 5, 125.
23. 23 R. G. Rubio, J. A. Zollweg and W. B. Streett, Ber. Bunsen-Ges. Phys. Chem., 1989, 93, 791.
24. 24 A. G. Aizpiri, A. Rey, J. Dávila and R. G. Rubio, J. Phys. Chem., 1991, 95, 3351.
25. 25 J. Ruthmann, S. A. Kovalenko and N. P. Ernsting, J. Chem. Phys., 1998, 109, 1.
26. 26 S. A. Kovalenko, H. Hennig, T. F. Laurent, N. P. Ernsting, T. A. Senyushkina and J. v. Frese, in preparation.
27. 27 B. M. Ladanyi and M. Maroncelli, J. Chem. Phys., 1998, 109, 3204.
28. 28 W. T. Lotshaw, D. McMorrow, N. Thantu, J. S. Melinger and R. Kitchenham, J. Raman Spectrosc., 1995, 26, 571.
29. 29 G. D. Patterson and J. E. Griffiths, J. Chem. Phys., 1975, 63, 2406.
30. 30 J. S. Friedman and C. Y. She, J. Chem. Phys., 1993, 99, 4960.
31. 31 D. McMorrow, W. T. Lotshaw and G. A. Kenney-Wallace, IEEE J. Quantum Electron, 1988, 24, 443.
32. 32 M. Cho, M. Du, N. F. Scherer, G. R. Fleming and S. Mukamel, J. Chem. Phys., 1993, 99, 2410.
33. 33 H. P. Deuel, P. Cong and J. D. Simon, J. Phys. Chem., 1994, 98, 12600.
34. 34 L. D. Ziegler, R. Fan, A. E. Desrosiers and N. F. Scherer, J. Chem. Phys., 1994, 100, 1823.
35. 35 S. Constantine, Y. Zhou, J. Morais and L. D. Ziegler, J. Phys. Chem. A, 1997, 101, 5456.
36. 36 Y. Zhou, S. Constantine, S. Harrel and L. D. Ziegler, J. Chem. Phys., 1999, 110, 5893.
37. 37 D. S. Alavi, R. S. Hartman and D. H. Waldeck, J. Chem. Phys., 1990, 92, 4055.
38. 38 G. C. Cho, W. Kütt and H. Kurz, Phys. Rev. Lett., 1990, 57, 321.
39. 39 M. J. Feldstein, P. Vöhringer and N. F. Scherer, J. Opt. Soc. Am. B, 1995, 12, 1500.
40. 40 D. A. Blank, L. J. Kaufman and G. R. Fleming., J. Chem. Phys., 1999, 111, 3105.
41. 41 Note that the sine transform of the model spike is irrelevant at low frequencies. It simply reflects the asymmetry of the model function at delays larger than the pulse width. There T(t) consists of several overlaid contributions and the model spike, when extended into this region, carries no meaning.
42. 42 Y. J. Chang and E. W. Castner, Jr., J. Chem. Phys., 1993, 99, 7289.
43. II(t) which may be related to corresponding nonequilibrium relaxation function. However in experimental spectroscopy it has become customary (see e.g. ref. 45) to apply the term "spectral density" to the imaginary part from the FT of the (nonequilibrium) response. Here we conform to this usage.
44. 44 W. H. Press, B. P. Flannery, S. A. Teukolsky and W. T. Vetterling, Numerical Recipes in Pascal. The Art of Scientific Computing, Cambridge University Press, Cambridge, 1990.
45. 45 P. Cong, J. D. Simon and C. Y. She, J. Chem. Phys., 1995, 104, 962.
46. -3, 100, 91}.
47. 47 Y. J. Yan and S. Mukamel, J. Chem. Phys., 1988, 89, 5160.
48. 48 H. Fröhlich, Theory of Dielectrics, Oxford University Press, London, 1958.
49. 49 B. N. Flanders, R. A. Cheville, D. Grischkowsky and N. F. Scherer, J. Phys. Chem., 1996, 100, 11824.
50. 50 E. W. Castner, Jr. and M. Maroncelli, J. Mol. Liq., 1998, 77, 1.
51. -1.
52. 52 B. M. Ladanyi and Y. Q. Liang, J. Chem. Phys., 1995, 103, 6325.
53. 53 S. Mukamel, A. Piryatinski and V. Chernyak, Acc. Chem. Res., 1999, 32, 145.
54. 54 J. Goulon, J. L. Rivail, J. W. Fleming, J. Chamberlain and G. W. Chantry, Chem. Phys. Lett., 1973, 18, 211.
55. 55 J. A. Riddick, W. B. Bunger and T. K. Sakano, Organic Solvents. Physical Properties and Methods of Purification, J. Wiley & Sons, New York, 1986.