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Omicron Vakuumphysik, Taunsstein, Germany
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Omicron Vakuumphysik, Taunsstein, Germany.
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6
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M. McEllistrem and J. J. Boland, in preparation
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M. McEllistrem and J. J. Boland, in preparation.
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10
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15144345614
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note
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2 was desorbed in a rapid anneal-and-quench thermal cycle, and the surface was imaged at room temperature. The rapid method minimizes the time available for the DBs to unpair, resulting in a population of predominantly paired DBs.
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12
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0000360045
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P. Nachtigall, K. D. Jordan, K. C. Janda, J. Chem. Phys. 95, 8652 (1991); M. P. D. D'Evelyn, Y. L. Yang, L. F. Sutcu, ibid. 98, 3560 (1993); U. Hofer, L. Li, T. F. Heinz, Phys. Rev. B 45, 9485 (1992).
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Nachtigall, P.1
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P. Nachtigall, K. D. Jordan, K. C. Janda, J. Chem. Phys. 95, 8652 (1991); M. P. D. D'Evelyn, Y. L. Yang, L. F. Sutcu, ibid. 98, 3560 (1993); U. Hofer, L. Li, T. F. Heinz, Phys. Rev. B 45, 9485 (1992).
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D'Evelyn, M.P.D.1
Yang, Y.L.2
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25544452706
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P. Nachtigall, K. D. Jordan, K. C. Janda, J. Chem. Phys. 95, 8652 (1991); M. P. D. D'Evelyn, Y. L. Yang, L. F. Sutcu, ibid. 98, 3560 (1993); U. Hofer, L. Li, T. F. Heinz, Phys. Rev. B 45, 9485 (1992).
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Hofer, U.1
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17
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J. H. G. Owen, D. R. Bowler, C. M. Goringe, K. Miki, G. A. D. Briggs, ibid. 54, 14153 (1996).
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Owen, J.H.G.1
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Briggs, G.A.D.5
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18
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0027724485
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In an earlier halogen study [J. J. Boland, Science 262, 1703 (1993)], we noted that at room temperature, two Cl atoms that were bonded on neighboring dimers showed a distinct preference to be on the same side of the dimer row. This preference remained even under imaging conditions where single Cl atoms (and unpaired DBs) readily hopped back and forth between sites on the same dimer.
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Boland, J.J.1
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19
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15144338671
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note
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A preliminary analysis of hopping rates to determine the relative energies of paired and unpaired configurations indicated that the predissociated configuration is stabilized compared with that of unpaired DBs, although not to the extent of paired DBs.
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21
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15144352789
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We thank E. J. Buehler and M. Fouchier for programming assistance, and M. Rubinstein and J. L. Whitten for insightful discussions. Financial support by NSF under contracts DMR 9509790 and DMR 9413999 is gratefully acknowledged.
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We thank E. J. Buehler and M. Fouchier for programming assistance, and M. Rubinstein and J. L. Whitten for insightful discussions. Financial support by NSF under contracts DMR 9509790 and DMR 9413999 is gratefully acknowledged.
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