Modeling the partial oxidation of methane in a short-contact-time reactor

AIChE Journal

Volumn 44, Issue 11, 1998, Pages 2465-2477

  Deutschmann, Olaf ^a,b   Schmidt, Lanny D ^a  

^a UNIVERSITY OF MINNESOTA   (United States)

^b UNIVERSITY OF HEIDELBERG   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

ALKANE; METHANE; METHANOL;

METHANE; NATURAL GAS; OXIDATION; REACTOR;

ARTICLE; ATMOSPHERIC PRESSURE; CATALYST; COMBUSTION; GAS; MATHEMATICAL MODEL; OXIDATION; PHASE TRANSITION; REACTOR; TEMPERATURE SENSITIVITY;

EID: 0032451186     PISSN: 00011541     EISSN: None     Source Type: Journal    
DOI: 10.1002/aic.690441114     Document Type: Article

References (14)

1. Bodke, A. S., and L. D. Schmidt, "The Effect of Ceramic Supports on Partial Oxidation of Hydrocarbons over Noble Metal Coated Monoliths," J. Catal., 179, 138 (1998).
2. Deuflhard, P., E. Hairer, and J. Zugk, "One-Step and Extrapolation Methods for Differential-Algebraic Systems," Num. Math., 51, 501 (1987).
3. Deutschmann, O., R. Schmidt, F. Behrendt, and J. Warnatz, "Numerical Modeling of Catalytic Ignition," Int. Symp. on Comb., p. 1747, Combust. Inst. (1996).
4. Deutschmann, O., F. Behrendt, and J. Warnatz, "Formal Treatment of Catalytic Conversion and Combustion of Methane," Catal. Today, in press (1998a).
5. Deutschmann, O., and L. D. Schmidt, "Two-Dimensional Modeling of Partial Oxidation of Methane on Rhodium in a Short Contact Time Reactor," Int. Symp. on Comb., Combustion Inst. (1998b).
6. Goetsch, D. A., and L. D. Schmidt, "Microsecond Catalytic Partial Oxidation of Alkanes," Science, 271, 1560 (1996).
7. 4 Oxidation on Pt and Rh Surfaces: High-Temperature Reactor Simulations," AIChE J., 39, 1164 (1993).
8. Hohn, K. L., P. M. Witt, M. B. Davis, and L. D. Schmidt, "Methane Coupling to Acetylene over Pt Coated Monoliths at Millisecond Contact Times," Catal. Lett., 54, 105 (1998).
9. Raja, L. L., R. J. Kee, and L. R. Petzold, "Simulation of the Transient, Compressible, Gas-Dynamic, Behavior of Catalytic-Combustion Ignition in Stagnation Flows," Int. Symp. on Comb., Combustion Inst. (1998).
10. Schmidt, L. D., O. Deutschmann, and C. T. Goralski, Jr., "Modeling the Partial Oxidation of Methane to Syngas at Millisecond Contact Times," Gas Conv. Symp., Taormina, Italy (Sept. 20-25, 1998).
11. Veser, G., J. Frauhammer, and L. D. Schmidt, "Catalytic Ignition of Methane Oxidation in a Monolithic Reactor," AIChE Meeting, Paper 266d, Los Angeles (Nov. 16-21, 1997).
12. Warnatz, J., M. D. Allendorf, R. J. Kee, and M. E. Coltrin, "A Model of Elementary Chemistry and Fluid Mechanics in the Combustion of Hydrogen on Platinum Surfaces," Combust. Flame, 96, 393 (1994).
13. Warnatz, J., "Hydrocarbon Oxidation Reaction Mechanism," personal communication (1998).
14. Witt, P. M., and L. D. Schmidt, "Effect of Flow Rate on the Partial Oxidation of Methane and Ethane," J. of Catal., 163, 465 (1996).