Acetylene hydrogenation on Ni-Al-Cr oxide catalysts: The role of added Zn

Applied Clay Science

Volumn 13, Issue 5-6, 1998, Pages 363-379

  Rives, V ^a   Labajos, F M ^a   Trujillano, R ^a   Romeo, E ^b   Royo, C ^b   Monzon A ^b  

^a UNIVERSITY OF SALAMANCA   (Spain)

^b UNIVERSITY OF ZARAGOZA   (Spain)

Author keywords

Acetylene hydrogenation; Cr doping; Hydrotalcite; Ni catalysts; Zn doping

Indexed keywords

CALCINATION; CATALYST ACTIVITY; CATALYST SELECTIVITY; CHROMIUM; CLAY MINERALS; COMPOSITION EFFECTS; DOPING (ADDITIVES); GAS ADSORPTION; HYDROGENATION; NICKEL ALLOYS; REDUCTION; ZINC;

HYDROTALCITE;

ACETYLENE;

ACETYLENE; CATALYSIS; HYDROTALCITE; ZINC;

EID: 0032214468     PISSN: 01691317     EISSN: None     Source Type: Journal    
DOI: 10.1016/S0169-1317(98)00033-7     Document Type: Article

References (36)

1. Al-Ubaid A., Wolf E.E. Steam reforming of methane on reduced non-stoichiometric nickel aluminate catalysts. Appl. Catal. 40:1988;73-85.
2. Arauzo J., Radlein D., Piskorz J., Scott D.S. A new catalyst for the catalytic gasification of biomass. Energy and Fuels. 8:1994;1192-1196.
3. 2 reforming of methane to syngas: Deactivation behavior of nickel aluminate spinel catalysts. Stud. Surf. Sci. and Catal. 88:1994;207-213.
4. Bradford M.C.J., Vannice M.A. Catalytic reforming of methane with carbon dioxide over nickel catalysts: I. Catalyst characterization and activity. Appl. Catal. A: General. 142:1996;73-96.
5. Bradford M.C.J., Vannice M.A. Catalytic reforming of methane with carbon dioxide over nickel catalysts: II. Reaction kinetics. Appl. Catal. A: General. 142:1996;97-122.
6. Cavani F., Trifiró F., Vaccari A. Hydrotalcite-type anionic clays: preparation, properties and applications. Catal. Today. 11(2):1991;173-301.
7. 3 interactions. Catal. Lett. 29:1994;39-48.
8. Clause O., Rebours B., Merlen E., Trifirò F., Vaccari A. Preparation and characterization of nickel-aluminum mixed oxides obtained by thermal decomposition of hydrotalcite-type precursors. J. Catal. 133:1992;231-246.
9. Courty Ph., Marcilly C. A scientific approach to the preparation of bulk mixed oxides. Stud. Surf. Sci. and Catal. 16:1983;485-519.
10. 6 alcohols from synthesis gas on copper-cobalt catalysts. J. Mol. Catal. 17:1982;241-254.
11. Edwards J.H., Maitra A.M. The chemistry of methane reforming with carbon dioxide and its current and potential applications. Fuel. Proc. Technology. 42:1995;269-289.
12. Fuda, K., Suda, K., Matsunaga, 1993. Oxidation of Cr(III) to Cr(VI) species during the thermal decomposition process of Zn/Cr-layered double hydroxide carbonate. Chem. Lett., 1479-1482.
13. Gusi S., Pizzoli F., Trifirò F., Vaccari A., del Piero G. Preparation of multicomponent catalysts for the hydrogenation of CO via hydrotalcite-like precursors. Stud. Surface Sci. Catal. 31:1987;753-765.
14. Huheey, J.E., 1983. Inorganic Chemistry: Principles of Structure and Reactivity, 3rd edn. Harper, Cambridge.
15. Jacobs J.P., Maltha A., Reintjes J.G.H., Drimal J., Ponec V., Brongersma H.H. The surface of catalytically active spinels. J. Catal. 147:1994;294-300.
16. Lobo L.S., Trimm D.L. Carbon formation from light hydrocarbons on nickel. J. Catal. 29:1973;15-19.
17. Malet P., Caballero A. The selection of experimental conditions in temperature-programmed reduction experiments. J. Chem. Soc., Faraday Trans. I. 84:1988;2369-2375.
18. Marchi, A.J., Di Cosimo, J.I., Apesteguía, C.R., 1988. Preparation of Cu-Co-Al mixed oxide catalysts for syngas conversion to higher alcohols. In: Phillips, M.J., Ternan, M. (Eds.), Proc. of the 9th International Congress on Catalysis, Vol. II. Calgary, Canada, pp. 529-536.
19. Marchi A.J., Di Cosimo J.I., Apesteguía C.R. Effect of preparation conditions on the reducibility of Cu-Co based oxides. Catal. Today. 15:1992;383-394.
20. Marchi A.J., Di Cosimo J.I., Apesteguía C.R. Influence of the chemical composition on the preparation of Cu-Co-Zn-Al mixed oxide catalysts with a high metal dispersion. Stud. Surf. Sci. and Catal. 75:1993;1171-1174.
21. Margitfalvi J., Guczi L., Weiss A.H. Reactions of acetylene during hydrogenation on Pd black catalyst. J. Catal. 72:1981;185-198.
22. Moses J.H., Weiss A.H., Matusek K., Guczi L. The effect of catalyst treatment on the selective hydrogenation of acetylene over palladium/alumina. J. Catal. 86:1984;417-426.
23. 4 catalyst. Stud. Surf. Sci. and Catal. 88:1994;555-560.
24. 4 catalyst: Characterization, coking and reaction studies. J. Catal. 159:1996;313-322.
25. Rives V., Ulibarri M.A., Montero A. Application of temperature-programmed reduction to the characterization of anionic clays. Appl. Clay Sci. 10:1995;83-93.
26. Rodríguez, J.C., 1996. Estudio de la Actividad, Selectividad y Estabilidad de Catalizadores de Hidrogenación Selectiva. PhD Thesis. Universidad de Zaragoza, Zaragoza, Spain, pp. 85-187.
27. Rodríguez J.C., Marchi A.J., Borgna A., Monzón A. Effect of Zn content on catalytic activity and physicochemical properties of Ni-based catalysts for selective hydrogenation of acetylene. J. Catal. 171:1997;268-278.
28. Rodríguez J.C., Guimon C., Marchi A., Borgna A., Monzón A. Activity, selectivity and coking of bimetallic Ni-Co-spinel catalysts in selective hydrogenation reactions. Stud. Surf. Sci. and Catal. 111:1997;183-190.
29. Ross J.R.H., Steel M.C.F., Zeini-Isfahani A. Evidence for the participation of surface nickel aluminate sites in the steam reforming of methane over nickel/alumina catalysts. J. Catal. 52:1978;280-290.
30. 3 como Catalizadores de Hidrogenación Selectiva. Abst. of the Xas Jornadas Argentinas de Catálisis, Buenos Aires, Argentina, pp. 415-417.
31. Somorjai, G.A., 1986. The building of catalysts: A molecular surface science approach. In: Hegedous, L.L. (Ed.), Catalyst Design. Progress and Perspectives. Wiley, New York, pp. 11-69.
32. Somorjai G.A., Carrazza J. Structure sensitivity of catalytic reactions. Ind. Eng. Chem. Fundam. 25:1986;63-69.
33. Somorjai G.A., Kesmodel L.L., Dubois L.H. LEED analysis of acetylene and ethylene chemisorption on the platinum (111) surface: evidence for ethylidine formation. J. Chem. Phys. 20:1979;2180-2188.
34. Tilley, R.J.D., 1987. Defect Crystal Chemistry and its Applications. Blackie and Sons, London.
35. Trifirò F., Vaccari A. Non-stoichiometry, a key to modify the activity and selectivity of spinel-type catalysts for hydrogenation reactions. Stud. Surf. Sci. and Catal. 67:1991;157-167.
36. Trifirò F., Vaccari A., Clause O. Nature and properties of nickel-containing mixed oxides obtained from hydrotalcite-type anionic clays. Catal. Today. 21:1994;185-195.