Ozonization of 2,4-dinitrotoluene and 4-nitroaniline as well as improved dissolved organic carbon removal by sequential ozonization-biodegradation

Water Environment Research

Volumn 70, Issue 2, 1998, Pages 146-154

  Saupe, Adrian ^a   Wiesmann, Udo ^a  

^a NONE

Author keywords

2,4 dinitrotoluene; 4 nitroaniline; Biodegradation; Chemical oxidation; Nitrate yield; Ozonization

Indexed keywords

AROMATIC HYDROCARBONS; BIODEGRADATION; MASS TRANSFER; METABOLITES; OXIDATION; OZONIZATION; PH EFFECTS; SUBSTRATES;

DINITROTOLUENE; DISSOLVED ORGANIC CARBON (DOC); NITROANILINE;

WASTEWATER TREATMENT;

2,4 DINITROTOLUENE; 4 NITROANILINE; AROMATIC NITRO COMPOUND; NITRATE; OZONE; UNCLASSIFIED DRUG;

ARTICLE; BIODEGRADATION; CONTROLLED STUDY; OXIDATION; PH; PRIORITY JOURNAL; WASTE WATER MANAGEMENT;

EID: 0032029486     PISSN: 10614303     EISSN: None     Source Type: Journal    
DOI: 10.2175/106143098X126982     Document Type: Article

References (44)

1. Andreozzi, R.; Caprio, V.; D'Amore, M.G.; and Insola, A. (1993) 1,2-Phenylenediamine Abatement in Aqueous Solution by Ozone. In Ozone in Water and Wastewater Treatment. Vol. 1, Proceedings of the Eleventh Ozone World Congress. San Francisco, Calif., 11-100.
2. Birou, B.; Ryhiner, G.; and Heinzle, E. (1994) Degradation of Recalcitrant Wastewater Components Combining Ozonation and Biological Treatment in a Novel Process Scheme. Proc. Int. Ozone Assoc. Reg. Conf., Zurich, Switz., 205.
3. Bradley P.M., and Chapelle, F.H. (1995) Factors Affecting Microbial 2,4,6-Trinitrotoluene Mineralization in Contaminated Soils. Environ. Sci. Technol., 29, 802.
4. Caprio, V., and Insola, A. (1985) Aniline and Anilinium Ion Ozonation in Aqueous Solution. Ozone Sci. Eng., 7, 167.
5. Chan, W.F., and Larson, R.A. (1991a) Mechanisms and Products of Ozonolysis of Aniline in Aqueous Solution Containing Nitrite Ion. Water Res. (G.B.), 25, 1539.
6. Chan, W.F., and Larson, R.A. (1991b) Formation of Mutagenes from the Aqueous Reactions of Ozone and Anilines. Water Res. (G.B.), 25, 1529.
7. Charpentier, J.C. (1981) Mass-Transfer Rates in Gas-Liquid Absorbers and Reactors. Adv. Chem. Eng., 11, 3.
8. Davis, E.M.; Murray, H.E.; Liehr, J.G.; and Powers, E.L. (1981) Basic Microbial Degradation Rates and Chemical Byproducts of Selected Organic Compounds. Water Res. (G.B.), 15, 1125.
9. Dickel, O., and Knackmuss, H.-J. (1991) Catabolism of 1,3-Dinitrobenzene by Rhodococcus sp. QT-1. Arch. Microbiol. (Ger.), 157, 76.
10. Dillert, R.; Brandt, M.; Fomefett, L; Siebers, U.; and Bahnemann, D. (1995) Photocatalytic Degradation of Trinitrotoluene and Other Nitroaromatic Compounds. Chemosphere, 30, 2333.
11. DIN 38 409 H 3-1 (1980) Summarische Wirkungs-und Stoffkenngrößen (Gruppe H). In Bestimmung des gesamten organisch gebundenen Kohlenstoffs (TOC). Beuth Verlag, Berlin, Ger.
12. DIN 38 409 H41 (1980) Summarische Wirkungs-und Stoffkenngrößen (Gruppe H). In Bestimmung des Chemischen Sauerstoff Bedarfs (CSB) im Bereich über 15 mg/L. Beuth Verlag, Berlin, Ger.
13. Franck, H.G., and Stadelhofer, J.W. (1987) Industrielle Aromatenchemie: Rohstoffe, Verfahren, Produkte. Springer Verlag, Berlin, Ger.
14. Fritsche, W., and Michels, J. (1996) Biologische Sanierung von Rüstungsaltlasten. BMBF-Verbundvorhaben, 2. Statusseminar, Jena, Ger.
15. Funk, St.B.; Roberts, D.J.; Crawford, D.L.; and Crawford, R.L. (1993) Initial-Phase Optimization for Bioremediation of Munition Compound-Contaminated Soils. Appl. Environ. Microbiol., 59, 2171.
16. Gilbert, E. (1987) Biodegradability of Ozonation Products as a Function of COD and DOC Elimination by Example of Substituted Aromatic Substances. Water Res. (G.B.), 21, 1273.
17. Gorontzy, T.; Drzyzga, O.; Kahl, M.W.; Bruns-Nagel, D.; Breitung, J.; von Loew, E.; and Blotevogel, K.-H. (1994) Microbial Degradation of Explosives and Related Compounds. Crit. Rev. Microbiol., 20, 265.
18. Haïdour, A., and Ramos, J.L. (1996) Identification of Products Resulting from the Biological Reduction of 2,4,6-Trinitrotoluene, 2,4-Dinitrotoluene and 2,6-Dinitrotoluene by Pseudomonas sp. Environ. Sci. Technol., 30, 2365.
19. Hallas, L.E., and Alexander, M. (1983) Microbial Transformation of Nitroaromatic Compounds in Sewage Effluent. Appl. Environ. Microbiol., 45, 1234.
20. Heinze, L.; Brosius, M.; and Wiesmann, U. (1995) Biologischer Abbau von 2,4-Dinitrotoluol in einer kontinuierlich betriebenen Versuchsanlage und kinetische Untersuchungen. Acta Hydrochim. Hydrobiol., 23, 254.
21. Heinzle, E.; Stockinger, H.; Stern, M.; Fahmy, M.; and Kut, O.M. (1995) Combined Biological-Chemical (Ozone) Treatment of Wastewaters Containing Chloroguaiacols. J. Chem. Tech. Biotechnol., 62, 241.
22. Ho, P.C. (1986) Photooxidation of 2,4-Dinitrotoluene in Aqueous Solution in the Presence of Hydrogen Peroxide. Environ. Sci. Technol., 20, 260.
23. Hoigné, J., and Bader, J. (1980) Bestimmung von Ozon und Chlordioxid in Wasser mit der Indigomethode. Vom Wasser (Ger.), 55, 261.
24. Hoigné, J.; Bader J.; Haag, W.R.; and Staehelin, J. (1985) Rate Constants of Reactions of Ozone with Organic and Inorganic Compounds in Water in, Inorganic Compounds and Radicals. Water Res. (G.B.), 19, 173.
25. Kaake, R.H.; Roberts, D.J.; Stevens, T.O.; Crawford, R.L.; and Crawford, D.L. (1992) Bioremediation of Soils Contaminated with the Herbicide 2-sec-Bury1-4,6-Dinitrophenol (Dinoseb). Appl. Environ. Microbiol., 58, 1683.
26. Kearney, Ph.C; Quiang Zeng; and Ruth, J.M. (1983) Oxidative Pretreatment Accelerates TNT Metabolism in Soils. Chemosphere, 17, 1583.
27. Langlais, B.; Cucurou, Y.A.; Capdeville, B.; and Roques, H. (1989) Improvement of a Biological Treatment by Prior Ozonation. Ozone Sci. Eng., 11, 155.
28. Lenke, H.; Daun, G.; Bryniok, D.; and Knackmuss, H.-J. (1993) Biologische Sanierung von Rüstungsaltlasten. Spektrum der Wissenschaft, 10/93, 106.
29. Lin, S.H., and Yen, Y.L. (1996) Ozonation Kinetics of Ammonia and Nitrite Removal From Aqueous Solution. J. Environ. Sci. Health, A31,4, 797.
30. Pasti-Grigsby, M.B.; Lewis, Th.A.; Crawford, D.L.; and Crawford, R.L. (1996) Transformation of 2,4,6-Trinitrotoluene (TNT) by Actinomycetes Isolated from TNT-Contaminated and Uncontaminated Environments. Appl. Environ. Microbiol., 61, 1120.
31. Rippen, G. (1991) Handbuch Umweltchemikalien * Stoffdaten * Prüfverfahren * Vorschriften, 3. Auflage. Ecomed Verlag, Berlin, Ger.
32. Roberts, DJ.; Ahmad, F.; and Pendharkar, S. (1996) Optimization of an Aerobic Polishing Stage to Complete the Anaerobic Treatment of Munition-Contaminated Soils. Environ. Sci. Technol., 30, 2021.
33. Ruppert, G., and Bauer, R. (1993) Mineralization of Cyclic Organic Water Contaminants by the Photo-Fenton Reaction Influence of Structure and Substituents. Chemosphere, 27, 1339.
34. 2 Slurries. Water Res. (G.B.), 29, 2651.
35. Scott, J.P., and Ollis, D.F. (1995) Integration of Chemical and Biological Oxidation Processes for Water Treatment: Review and Recommendations. Environ. Prog., 14, 88.
36. Spanggord, R.J.; Gibson, B.W.; Keck, R.G.; and Thomas, D.W. (1982) Effluent Analysis of Wastewater Generated in the Manufacture of 2,4,6-Trinitrotoluene. 1. Characterization Study. Environ. Sci. Technol., 16, 229.
37. Stem, M.; Heinzle, E.; Kut, O.M.; and Hungerbühler, K. (1996) Removal of Substituted Pyridines by Combined Ozonization/Fluidized Bed Biofilm Treatment. Paper presented at Int. Conf. Oxidation Technol. Water Wastewater 1996, CUTEC Schriftenreihe Nr. 23, Clausthal-Zellerfeld, A. Vogelpohl (Ed.), Goslar, Ger.
38. Stockinger, G. (1995) Removal of Biorefractory Pollutants in Wastewater by Combined Ozonation-Biotreatment. Doctoral diss., Eidgenössische Technische Hochschule, ETH No. 11063, Zurich, Switz.
39. 3-N. Tecator Company, Swed.
40. Valli, K.; Brock, B.J.; Joshi, D.; and Gold, M.H. (1992) Degradation of 2,4-Dinitrotoluene by the Lignin-Degrading Fungus Phanerochaete chrysosporium. Appl. Environ. Microbiol., 58, 221.
41. Wang, B., and Yin, J. (1988) Removal of Aromatic Nitro Compounds from Water by Ozonation. Ozone Sci. Eng., 10, 1.
42. Xu, S.-C; Zhou, H.-D.; Wei, X.-Y.; and Lu, J. (1989) The pH Dependence and Effects of the Oxidative Products of Some Aromatic Compounds in Ozonation under UV Irradiation. Ozone Sci. Eng., 11, 281.
43. Yinon, J. (1990) Toxicity and Metabolism of Explosives. CRC Press, Boca Raton, Fla.
44. 14C]-Carbon Dioxide. J. Agric. Food Chem., 31, 304.