Off-resonant coherent hyper-Raman scattering spectroscopy

Journal of Chemical Physics

Volumn 106, Issue 18, 1997, Pages 7550-7557

  Cho, Minhaeng ^a  

^a Korea University   (South Korea)

Author keywords

[No Author keywords available]

Indexed keywords

HAMILTONIANS; RAMAN SCATTERING; APPROXIMATION THEORY; ELECTRON ENERGY LEVELS; LASER PULSES; LIGHT POLARIZATION; MATHEMATICAL MODELS; NATURAL FREQUENCIES;

EFFECTIVE HAMILTONIAN; HETERODYNE METHOD; HYPER-RAMAN; MACROSCOPIC POLARIZATION; MEASURED SIGNALS; PUMP FIELDS; SCATTERING SIGNALS; TRANSIENT GRATING;

COHERENT SCATTERING; RAMAN SPECTROSCOPY;

CHROMOPHORES; COHERENT HYPER RAMAN SCATTERING SPECTROSCOPY; HAMILTONIAN; HETERODYNE SIGNAL; HOMODYNE SIGNAL; LIOUVILLE EQUATIONS;

EID: 0031559337     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.473758     Document Type: Article

References (26)

1. N. Bloembergen, Nonlinear Optics (Benjamin, New York, 1965).
2. Y. R. Shen, The Principles of Nonlinear Optics (Wiley, New York, 1984).
3. M. D. Levenson and S. S. Kano, Introduction to Nonlinear Laser Spectroscopy (Academic, New York, 1988).
4. P. N. Butcher and D. Cotter, The Elements of Nonlinear Optics (Cambridge University Press, Cambridge, 1990).
5. S. Mukamel, Principles of Nonlinear Optical Spectroscopy (Oxford, New York, 1995).
6. G. R. Fleming, Chemical Applications of Ultrafast Spectroscopy (Oxford, New York, 1986).
7. G. R. Fleming and M. Cho, Ann. Rev. Phys. Chem. 47, 109 (1996).
8. Ultrafast Laser Pulses and Applications, edited by W. Kaiser, Topics in Applied Physics, Vol. 60 (Springer, Berlin, 1988).
9. Nonlinear Optical Properties of Organic Molecules and Crystals, edited by D. S. Chemla and J. Zyss (Academic, Orlando, 1987).
10. S. R. Marder, C. B. Gorman, F. Meyers, J. W. Perry, G. Bourhill, J.-L. Brédas, and B. M. Pierce, Science, 265, 632 (1994).
11. D. Yaron and R. J. Silbey, Phys. Rev. B 45, 11 655 (1992).
12. I. D. W. Samuel, I. Ledoux, C. Dhenaut, J. Zyss, H. H. Fox, R. R. Schrock, and R. J. Silbey, Science 265, 1070 (1994).
13. C. Castinglioni, M. Del Zoppo, and G. Zerbi, Phys. Rev. B 53, 13 319 (1996).
14. D. Lu, G. Chen, J. W. Perry, and W. A. Goddard III, J. Am. Chem. Soc. 116, 10 679 (1994).
15. G. Chen and S. Mukamel, J. Chem. Phys. 103, 9355 (1995).
16. D. N. Beratan, J. N. Onuchic, and J. W. Perry, J. Phys. Chem. 91, 2696 (1987).
17. B. F. Levine and C. G. Bethea, J. Chem. Phys. 65, 2429 (1976).
18. K. Clays and A. Persoons, Phys. Rev. Lett. 66, 2980 (1991).
19. S. Mukamel and R. F. Loring, J. Opt. Soc. Am. B 3, 595 (1986).
20. M. Cho, M. Du, N. F. Scherer, G. R. Fleming, and S. Mukamel, J. Chem. Phys. 99, 2410 (1993).
21. Y . X. Yan and K. A. Nelson, J. Chem. Phys. 87, 6240 (1987).
22. S. Mukamel, Adv. Chem. Phys. 70, 165 (1988).
23. One can prove that this approximation is quite reasonable in the case of an off-resonant excitation field, by calculating the transition probability perturbatively (refer to Ref. 20 for detailed discussion for a two-state system showing optical Kerr effect).
24. M. D. Fayer, Ann. Rev. Phys. Chem. 33, 63 (1982).
25. Y. J. Yan and S. Mukamel, J. Chem. Phys. 94, 997 (1991).
26. L. D. Landau and E. M. Lifshitz, Statistical Physics, Part I, (Pergamon, Oxford, 1963).