The role of local density in the collisional deactivation of vibrationally highly excited azulene in supercritical fluids

Journal of Chemical Physics

Volumn 107, Issue 20, 1997, Pages 8380-8390

  Schwarzer, D ^a   Troe, J ^a   Zerezke, M ^a  

^a MAX PLANCK INSTITUTE FOR BIOPHYSICAL CHEMISTRY   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

COMPUTER SIMULATION; DENSITY (SPECIFIC GRAVITY); ENERGY TRANSFER; LASER APPLICATIONS; LIGHT ABSORPTION; MATHEMATICAL MODELS; MOLECULES; MONTE CARLO METHODS; PHASE TRANSITIONS; SOLVENTS; SPECTROSCOPY;

AZULENE; COLLISIONAL DEACTIVATION; ISOLATED BINARY COLLISION; LASER EXCITATION; LENNARD-JONES FLUID; PUMP AND PROBE PICOSECOND LASER SPECTROSCOPY; SOLVATOCHROMIC SHIFT; SUPERCRITICAL FLUID;

PHOTOCHEMICAL REACTIONS;

EID: 0031273077     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.475038     Document Type: Article

References (69)

1. M. Quack and J. Troe, in Gas Kinetics and Energy Transfer, edited by P. G. Ashmore and R. J. Donovan (The Chemical Society, London, 1977), Vol. 2, p. 175; H. Hippler and J. Troe, in Bimolecular Collisions, edited by M. N. R. Ashfold and J. E. Baggott (The Royal Society of Chemistry, London, 1989), p. 209.
2. M. Quack and J. Troe, in Gas Kinetics and Energy Transfer, edited by P. G. Ashmore and R. J. Donovan (The Chemical Society, London, 1977), Vol. 2, p. 175; H. Hippler and J. Troe, in Bimolecular Collisions, edited by M. N. R. Ashfold and J. E. Baggott (The Royal Society of Chemistry, London, 1989), p. 209.
3. D. C. Tardy and B. S. Rabinovitch, Chem. Rev. 77, 396 (1977); I. Oref and D. C. Tardy, ibid. 90, 1407 (1990).
4. D. C. Tardy and B. S. Rabinovitch, Chem. Rev. 77, 396 (1977); I. Oref and D. C. Tardy, ibid. 90, 1407 (1990).
5. H. Hippler, J. Troe, and H. J. Wendelken, Chem. Phys. Lett. 84, 257 (1981); J. Chem. Phys. 78, 6709 (1983).
6. H. Hippler, J. Troe, and H. J. Wendelken, Chem. Phys. Lett. 84, 257 (1981); J. Chem. Phys. 78, 6709 (1983).
7. H. Hippler, K. Luther, and J. Troe, J. Chem. Phys. 78, 6718 (1983); M. Damm, H. Hippler, and J. Troe, ibid. 88, 3564 (1988).
8. H. Hippler, K. Luther, and J. Troe, J. Chem. Phys. 78, 6718 (1983); M. Damm, H. Hippler, and J. Troe, ibid. 88, 3564 (1988).
9. M. Heymann, H. Hippler, D. Nahr, H. J. Plach, and J. Troe, J. Phys. Chem. 92, 5507 (1988); J. E. Dove, H. Hippler, H. J. Plach, and J. Troe, J. Chem. Phys. 81, 1209 (1984).
10. M. Heymann, H. Hippler, D. Nahr, H. J. Plach, and J. Troe, J. Phys. Chem. 92, 5507 (1988); J. E. Dove, H. Hippler, H. J. Plach, and J. Troe, J. Chem. Phys. 81, 1209 (1984).
11. H. Hippler, B. Otto, and J. Troe, Ber. Bunsenges. Phys. Chem. 93, 428 (1989).
12. G. P. Smith and J. R. Barker, Chem. Phys. Lett. 78, 253 (1981); J. Shi, D. Bernfeld, and J. R. Barker, J. Chem. Phys. 88, 6211 (1988); J. Shi and J. R. Barker, ibid. 88, 6219 (1988).
13. G. P. Smith and J. R. Barker, Chem. Phys. Lett. 78, 253 (1981); J. Shi, D. Bernfeld, and J. R. Barker, J. Chem. Phys. 88, 6211 (1988); J. Shi and J. R. Barker, ibid. 88, 6219 (1988).
14. G. P. Smith and J. R. Barker, Chem. Phys. Lett. 78, 253 (1981); J. Shi, D. Bernfeld, and J. R. Barker, J. Chem. Phys. 88, 6211 (1988); J. Shi and J. R. Barker, ibid. 88, 6219 (1988).
15. B. M. Toselli, J. D. Brenner, M. L. Yarram, W. E. Chin, K. D. King, and J. R. Barker, J. Chem. Phys. 95, 176 (1991).
16. U. Hold, T. Lenzer, K. Luther, K. Reihs, and A. Symonds. Ber. Bunsenges. Phys. Chem. 101, 552 (1997).
17. J. Troe, J. Chem. Phys. 77, 3485 (1982); J. R. Barker, J. Phys. Chem. 88, 11 (1984).
18. J. Troe, J. Chem. Phys. 77, 3485 (1982); J. R. Barker, J. Phys. Chem. 88, 11 (1984).
19. K. F. Lim and R. G. Gilbert, J. Chem. Phys. 80, 5501 (1984); 84, 6129 (1986).
20. K. F. Lim and R. G. Gilbert, J. Chem. Phys. 80, 5501 (1984); 84, 6129 (1986).
21. A. J. Stace and J. N. Murrell, J. Chem. Phys. 68, 3028 (1978); N. J. Brown and J. A. Miller, ibid. 80, 5568 (1984): H. Hippler, H. W. Schranz, and J. Troe, J. Phys. Chem. 40, 6158 (1986).
22. A. J. Stace and J. N. Murrell, J. Chem. Phys. 68, 3028 (1978); N. J. Brown and J. A. Miller, ibid. 80, 5568 (1984): H. Hippler, H. W. Schranz, and J. Troe, J. Phys. Chem. 40, 6158 (1986).
23. A. J. Stace and J. N. Murrell, J. Chem. Phys. 68, 3028 (1978); N. J. Brown and J. A. Miller, ibid. 80, 5568 (1984): H. Hippler, H. W. Schranz, and J. Troe, J. Phys. Chem. 40, 6158 (1986).
24. M. Bruehl and G. Schatz, J. Phys. Chem. 42, 7223 (1988).
25. Th. Lenzer, K. Luther, J. Troe, R. G. Gilbert, and K. F. Lim, J. Chem. Phys. 103, 626 (1995).
26. F. Wondrazek, A. Seilmeier, and W. Kaiser, Chem. Phys. Lett. 104, 121 (1984).
27. A. Seilmeier, P. O. J. Scherer, and W. Kaiser, Chem. Phys. Lett. 105, 140 (1984).
28. U. Sukowski, A. Seilmeier, T. Elsaesser, and S. F. Fischer, J, Chem. Phys. 93, 4094 (1990).
29. H. Miyasaka, M. Hagihara, T. Okada. and N. Malaga, Chem. Phys. Lett. 188, 259 (1992).
30. K. E. Schultz, D. J. Russel, and C. B. Harris, J. Chem. Phys. 97, 5431 (1992).
31. R. J. Sension, S. T. Repinec, A. Z. Szarka, and R. M. Hochstrasser, J. Chem. Phys. 98, 6291 (1993).
32. K. Lenz, M. Pfeiffer, A. Lau, and T. Elsaesser, Chem. Phys. Lett. 229, 340 (1994).
33. T. Elsaesser and W. Kaiser, Annu. Rev. Phys. Chem. 42, 83 (1991).
34. D. Schwarzer, J. Troe, M. Votsmeier, and M. Zerezke, J. Chem. Phys. 105, 3121 (1996).
35. J. Benzler, S. Linkersdörfer, and K. Luther. Ber. Bunsenges. Phys. Chem. 100, 1252 (1996).
36. D. Schwarzer, J. Troe, M. Votsmeier, and M. Zerezke, Ber. Bunsenges. Phys. Chem. 101, 595 (1997).
37. (a) C. A. Eckert, D. H. Ziger, K. P. Johnston, and T. K. Ellison, Fluid Phase Equilibria 14, 167 (1983)
38. (b) C. A. Eckert, D. H. Ziger, K. P. Johnston, and S. Kim, J. Phys. Chem. 90, 2738 (1986).
39. S. Kim and K. P. Johnston, Ind. Eng. Chem. Res. 26, 1206 (1987); G. E. Bennett and K. P. Johnston, J. Phys. Chem. 98. 441 (1994); O. Kajimoto, M. Futakami, T. Kobayashi, and K. Yamasaki, ibid. 92, 1347 (1988); A. Morita and O. Kajimoto, ibid. 94, 6420 (1990).
40. S. Kim and K. P. Johnston, Ind. Eng. Chem. Res. 26, 1206 (1987); G. E. Bennett and K. P. Johnston, J. Phys. Chem. 98. 441 (1994); O. Kajimoto, M. Futakami, T. Kobayashi, and K. Yamasaki, ibid. 92, 1347 (1988); A. Morita and O. Kajimoto, ibid. 94, 6420 (1990).
41. S. Kim and K. P. Johnston, Ind. Eng. Chem. Res. 26, 1206 (1987); G. E. Bennett and K. P. Johnston, J. Phys. Chem. 98. 441 (1994); O. Kajimoto, M. Futakami, T. Kobayashi, and K. Yamasaki, ibid. 92, 1347 (1988); A. Morita and O. Kajimoto, ibid. 94, 6420 (1990).
42. S. Kim and K. P. Johnston, Ind. Eng. Chem. Res. 26, 1206 (1987); G. E. Bennett and K. P. Johnston, J. Phys. Chem. 98. 441 (1994); O. Kajimoto, M. Futakami, T. Kobayashi, and K. Yamasaki, ibid. 92, 1347 (1988); A. Morita and O. Kajimoto, ibid. 94, 6420 (1990).
43. Y. Sun, G. Bennett, K. P. Johnston, and M. A. Fox, J. Phys. Chem. 96, 10001 (1992).
44. P. G. Debenedetti, Chem. Eng. Sci. 42, 2203 (1987).
45. I. B. Petsche and P. G. Debenedetti, J. Chem. Phys 91, 7075 (1989).
46. R. S. Urdahl, K. D. Rector, D. J. Myers, P. H. Davis, and M. D. Fayer, J. Chem. Phys. 105, 8973 (1996).
47. D. Schwarzer, J. Troe, and J. Schroeder, Ber. Bunsenges. Phys. Chem. 95, 933 (1991); B. D. Wagner, M. Szymanski, and R. P. Steer, J. Chem. Phys. 98, 301 (1993).
48. D. Schwarzer, J. Troe, and J. Schroeder, Ber. Bunsenges. Phys. Chem. 95, 933 (1991); B. D. Wagner, M. Szymanski, and R. P. Steer, J. Chem. Phys. 98, 301 (1993).
49. Th. Bultmann, D. Bingemann, N. Ernsting, D. Schwarzer, and L. Nikowa, Rev. Sci. Instrum. 66, 4393 (1995).
50. L. Brouwer, H. Hippler, L. Lindemann, and J. Troe, J. Phys. Chem. 89, 4608 (1985).
51. H, Hippler, L. Lindemann, and J. Troe, J. Chem. Phys. 83, 3906 (1985).
52. Messer Griesheim, Physical Properties of Gases, Sach-Nr. 0.812.251, ed. 8109/VII.
53. B. A. Younglove and J. F. Ely, J. Phys. Chem. Ref. Data 16, 577 (1987).
54. D. G. Friend, H. Ingham, and J. F. Ely, J. Phys. Chem. Ref. Data 20, 257 (1991).
55. J. Chesnoy and G. M. Gale, Ann. Phys. (Paris) 9, 893 (1984).
56. T. Einwohner and B. J. Alder, J. Chem. Phys. 49, 1458 (1968).
57. P. K. Davis and I. Oppenheim, J. Chem. Phys. 57, 505 (1972).
58. C. Delalande and G. M. Gale, J. Chem. Phys. 71, 4804 (1979).
59. R. C. Reid, J. M. Prausnitz, and T. K. Sherwood, The Properties of Gases and Liquids, 3rd ed. (McGraw-Hill, New York, 1977).
60. N. Metropolis, A. W. Rosenbluth, M. N. Rosenbluth, A. H. Teller, and E. Teller, J. Chem. Phys. 21, 1087 (1953).
61. M. P. Allen and D. J. Tildesley, Computer Simulations of Liquids (Oxford University Press, Oxford, 1987).
62. D. A. McQuarrie Statistical Mechanics (Harper & Row, New York, 1973).
63. E. G. McRae, J. Phys. Chem. 61, 562 (1957).
64. E. Lippert, Ber. Bunsenges. Phys. Chem. 61, 562 (1957)
65. W. Liptay, in Modern Quantum Chemistry, edited by O. Sinanoglu (Academic, New York, 1966), Part II, p. 173.
66. T. Abe, Bull. Chem. Soc. Jpn. 38, 1314 (1965).
67. H. Margenau, Rev. Mod. Phys. 11, 1 (1939).
68. A. T. Amos and B. L. Burrows, Adv. Quantum Chem. 7, 289 (1973).
69. A. Z. Panagiotopoulos, Mol. Phys. 61, 813 (1987).