Surface chemistry of alkyl and perfluoro ethers: A FTIR and ab initio study of adsorption and decomposition of CF3OCF3 on an Al2O3 surface

Surface Science

Volumn 380, Issue 2-3, 1997, Pages 530-539

  Li, Ping ^a   Ng, L M ^a   Liang, Jim ^b  

^a CLEVELAND STATE UNIVERSITY   (United States)

^b UNIVERSITY OF DAYTON RESEARCH INSTITUTE   (United States)

Author keywords

Ab initio quantum chemical methods and calculations; Aluminum oxide; Catalysis; Fluorinated ethers; Fluoroformate; Infrared adsorption spectroscopy; Polycrystalline surfaces; Surface chemical reaction

Indexed keywords

ADSORPTION; ALUMINA; CATALYSIS; FOURIER TRANSFORM INFRARED SPECTROSCOPY; POLYCRYSTALLINE MATERIALS; PYROLYSIS; REACTION KINETICS; THERMAL EFFECTS;

PERFLUORODIMETHYL ETHERS;

ETHERS;

EID: 0031142101     PISSN: 00396028     EISSN: None     Source Type: Journal    
DOI: 10.1016/S0039-6028(97)00037-X     Document Type: Article

References (27)

1. J.F. Moulder, J.S. Hammond and K.L. Smith, Appl. Surf. Sci. 25 (1986) 446.
2. C.E. Snyder, Jr., and R.E. Dolle. Jr., ASLE Trans. 19 (1976) 171.
3. P.H. Kasai, W.T. Tang and P. Wheeler, Appl. Surf. Sci. 51 (1991) 201.
4. M.M. Walczak, P.K. Leavitt and P.A. Thiel, J. Am. Chem. Soc. 109 (1987) 5621.
5. V. Maurice, K. Takeuchi, M. Salmeron and G.A., Somorjai, Surf. Sci. 250 (1991) 99.
6. L.M. Ng, E. Lyth, M.V. Zeller and D.L. Boyd, Langmuir 11 (1995) 127.
7. E. Lyth and L.M. Ng, J. Phys. Chem. 99 (1995) 17615.
8. D.A. Munro and L.M. Ng, Langmuir, 12 (1996) 739.
9. P. Li and L.M. Ng, Surf. Sci. 342 (1995) 359.
10. M.M. Walczak and P.A. Thiel, Surf. Sci. 17 (1989) 89.
11. H. Bürger and G. Pawelke. Spectrochim. Acta A 31 (1975) 1165.
12. J.D. Witt, J.R. Durig, D. DesMarteau and R.M. Hammaker, Inorg. Chem. 12 (1973) 807.
13. J.B. Peri, J. Phys. Chem. 69 (1965) 211.
14. J.B. Peri and R.B. Hannan, J. Phys. Chem. 64 (1960) 1526.
15. J.G. Chen, P. Basu, T.H. Ballinger and J.T. Yates, Jr., Langmuir, 5 (1989) 352.
16. J. Pacansky, M. Miller, W. Hatton, B. Liu and A. Scheiner, J. Am. Chem. Soc. 113 (1991) 329.
17. G. Busca, J. Lamotte. J.-C. Lavalley and V. Lorenzelli, J. Am. Chem. Soc. 109 (1987) 5197.
18. P.G. Gopal. R.L. Schneider and K.L. Watters. J. Catal. 105 (1987) 366.
19. B.S. Ault, Inorg. Chem. 21 (1982) 756.
20. M.J. Frisch, G.W. Trucks, H.B. Schlegel. P.M.W. Gill, B.G. Johnson, M.W. Wong, J.B. Foresman, M.A. Robb, M. Head-Gordon. E.S. Replogle, R. Gomperts, J.L. Andres, K. Raghavachari, J.S. Binkley, C. Gonzalez, R.L. Martin, D.J. Fox, D.J. Defrees, J. Baker, J.J.P. Stewart and J.A. Pople, Gaussian 92 DFT, Revision G.3 (Gaussian, Inc., Pittsburgh PA, 1993); M.J. Frisch, G.W. Trucks, H.B. Schlegel, P.M.W. Gill, B.G. Johnson, M.A. Robb, J.R. Cheeseman, T. Keith, G.A. Petersson, J.A. Montgomery. K. Raghavachari, M.A. Al-Laham, V.G. Zakrzewski, J.V. Ortiz, J.B. Foresman, J. Cioslowski, B.B. Stefanov, A. Nanayakkara, M. Challacombe, C.Y. Peng, P.Y. Ayala, W. Chen. M.W. Wong, J.L. Andres, E.S. Replogle, R. Gomperts, R.L. Martin, D.J. Fox, J.S. Binkley, D.J. Defrees, J. Baker, J.P. Stewart, M. Head-Gordon, C. Gonzalez and J.A. Pople, Gaussian 94, Revision C.3 (Gaussian Inc., Pittsburgh PA, 1995).
21. M.J. Frisch, G.W. Trucks, H.B. Schlegel. P.M.W. Gill, B.G. Johnson, M.W. Wong, J.B. Foresman, M.A. Robb, M. Head-Gordon. E.S. Replogle, R. Gomperts, J.L. Andres, K. Raghavachari, J.S. Binkley, C. Gonzalez, R.L. Martin, D.J. Fox, D.J. Defrees, J. Baker, J.J.P. Stewart and J.A. Pople, Gaussian 92 DFT, Revision G.3 (Gaussian, Inc., Pittsburgh PA, 1993); M.J. Frisch, G.W. Trucks, H.B. Schlegel, P.M.W. Gill, B.G. Johnson, M.A. Robb, J.R. Cheeseman, T. Keith, G.A. Petersson, J.A. Montgomery. K. Raghavachari, M.A. Al-Laham, V.G. Zakrzewski, J.V. Ortiz, J.B. Foresman, J. Cioslowski, B.B. Stefanov, A. Nanayakkara, M. Challacombe, C.Y. Peng, P.Y. Ayala, W. Chen. M.W. Wong, J.L. Andres, E.S. Replogle, R. Gomperts, R.L. Martin, D.J. Fox, J.S. Binkley, D.J. Defrees, J. Baker, J.P. Stewart, M. Head-Gordon, C. Gonzalez and J.A. Pople, Gaussian 94, Revision C.3 (Gaussian Inc., Pittsburgh PA, 1995).
22. B.C. Lippens and J.J. Steggerda, in: Physical and Chemical Aspects of Adsorbents and Catalysts, Eds. B.G. Linsen et al. (Academic. London and New York. 1970) p. 171.
23. A.P. Borosy. B. Silvi, M. Allavena and P. Nortier, J. Phys. Chem. 98 (1994) 13189.
24. Hisayoshi Kobayashi, Masaru Yamaguchi, Tsunehiro Tanaka. Yasuo Nishimura. Hiroshi Kawakami and Satohiro Yoshida, J. Phys. Chem. 92 (1988) 2516.
25. CRC Handbook of Chemistry and Physics, 73rd ed., Ed. David R. Lide (CRC, Boca Raton, Ann Arbor. London, Tokyo, 1992) p. 9.
26. J.B. Foresman and E. Frisch. Exploring Chemistry with Electronic Structure Methods: A Guide to using Gaussian, 1st edn. (Gaussian, Inc., Pittsburgh, PA. 1993).
27. J.E. Crowell, J.G. Chen and J.T. Yates, Jr. J. Chem. Phys. 85 (1986) 3111.