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3643080786
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note
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Similar kinetics has also been reported for the phenomenon of lamellar thickening in poly(ethylene) and other flexible polymers. However, lamellar thickening is accompanied by an increase in long spacing, and the underlying physical processes are very different from the processes that accompany the development of the low endotherm in semiflexible semicrystalline polymers. Therefore, we have deliberately not cited the kinetics of lamellar thickening.
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16
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3643115170
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note
-
In the past, some of us proposed a model that was completely different from the models discussed in the text. We proposed that the low endotherm is the enthalpic recovery of a physically aged rigid amorphous fraction. We now acknowledge that we were in error. Therefore, we will not dwell on that explanation in the text.
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85088542278
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26 this corresponds to the development of the high endotherm and not the low endotherm.
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3643103704
-
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note
-
The dimensions for the liquid pockets are quoted for high crystallization temperatures only. For lower crystallization temperatures, we expect the average size of the liquid pockets to be lower.
-
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-
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45
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0000596095
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50
-
-
85088542396
-
-
note
-
cl are both constant. Therefore, eq 8 can be assumed to be valid only in a limited temperature range just above the glass transition.
-
-
-
-
51
-
-
3643063022
-
-
in preparation
-
Verma, R. K.; Velikov, V.; Marand, H.; Sauer, B. B.; Dee, G. T., in preparation.
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Verma, R.K.1
Velikov, V.2
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52
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0024639812
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57
-
-
3643116255
-
-
note
-
The cited number was obtained from a visual estimate of Figure 3 in ref 56.
-
-
-
-
58
-
-
3643119333
-
-
See, for instance, Figure 3 in ref 52
-
See, for instance, Figure 3 in ref 52.
-
-
-
-
59
-
-
3643067248
-
-
note
-
In eq 9, we are treating the isothermal compressibility κ as independent of pressure. This is not strictly true (see, for instance, eq 6 in ref 52). Therefore, eq 9 is an approximation which we use only for illustration.
-
-
-
-
60
-
-
85088544597
-
-
note
-
ρamorphous was then calculated from Table II of ref 52 and verified with our own work of ref 51. While the exact values may differ somewhat, the final calculations are, for the most part, unaffected by slight variations in the exact values.
-
-
-
-
61
-
-
85088543750
-
-
note
-
c relaxation.
-
-
-
-
63
-
-
3643061991
-
-
note
-
cl from the correlation function). However, we expect the average lamellar thickness to be altered somewhat in the drawn samples.
-
-
-
-
64
-
-
0026832211
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Lovinger, A. J.; Hudson, S. D.; Davis, D. D. Macromolecules 1992, 25, 1752.
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Lovinger, A.J.1
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Davis, D.D.3
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