Temporal variations in formaldehyde, acetaldehyde and acetone and budget of formaldehyde at a rural site in southern Germany

Atmospheric Environment

Volumn 30, Issue 21, 1996, Pages 3667-3676

  Slemr, J ^a   Junkermann, W ^a   Volz Thomas, A ^b  

^a KARLSRUHE INSTITUTE OF TECHNOLOGY   (Germany)

^b FORSCHUNGSZENTRUM JÜLICH   (Germany)

Author keywords

Acetaldehyde; Acetone; Emission; Formaldehyde; Photochemistry; Transport; Troposphere

Indexed keywords

ACETALDEHYDE; ACETONE; FORMALDEHYDE;

AIR POLLUTION; ARTICLE; COVARIANCE; ENVIRONMENTAL MONITORING; FLUOROMETRY; GERMANY; NIGHT; PHOTOCHEMISTRY; PRIORITY JOURNAL; RURAL AREA; TROPOSPHERE;

ACETALDEHYDE; ACETONE; ATMOSPHERIC TRANSPORT; FORMALDEHYDE; MIXING RATIO; PHOTOCHEMISTRY; RURAL AREA; TEMPORAL VARIATION; TRACT; TROPOSPHERE;

GERMANY, SAARLAND, SCHAUINSLAND;

ACETONE; AIR POLLUTION; ATMOSPHERIC COMPOSITION; HIGH PRESSURE LIQUID CHROMATOGRAPHY; METEOROLOGY; MIXING; PHOTOCHEMICAL REACTIONS; SAMPLING; TROPOSPHERE;

ACETALDEHYDE; GERMANY; MIXING RATIOS; MOLE FRACTIONS;

FORMALDEHYDE;

EID: 0030274171     PISSN: 13522310     EISSN: None     Source Type: Journal    
DOI: 10.1016/1352-2310(96)00025-8     Document Type: Article

References (39)

1. Altshuller A. P. (1991a) Chemical reactions and transport of alkanes and their products in the troposphere. J. atmos. Chem. 12, 19-61.
2. Altshuller A. P. (1991b) Estimating product yields of carbon-containing products from the atmospheric photooxidation of ambient air alkenes. J. atmos. Chem. 13, 131-154.
3. Altshuller A. P. (1993) Production of aldehydes as primary emissions and from secondary atmospheric reactions of alkenes and alkanes during the night and early morning hours. Atmospheric Environment 27A, 21-32.
4. Atkinson R. (1990) Gas-phase tropospheric chemistry of organic compounds: a review. Atmospheric Environment 24A, 1-41.
5. Brunke E.-G. (1988) Influence of guano beds on the tropospheric formaldehyde level in marine air at Cape Point. South African J. Sci. 84, 118-121.
6. Carlier P., Hannachi H. and Mouvier G. (1986) The chemistry of carbonyl compounds in the atmosphere - a review. Atmospheric Environment 20, 2079-2099.
7. Chatfield R. B., Gardner E. P. and Calvert J. G. (1987) Sources and sinks of acetone in the troposphere: behaviour of reactive hydrocarbons and a stable product. J. geophys. Res. 92, 4208-4216.
8. Cleveland W. S., Graedel T. E. and Kleiner B. (1977) Urban formaldehyde: observed correlation with source emissions and photochemistry. Atmospheric Environment 11, 357-360.
9. Dodge M. (1990) Formaldehyde production in photochemical smog as predicted by three state-of-the-science chemical oxidant mechanisms. J. geophys. Res. 95, 3635-3648.
10. Fehsenfeld F., Calvert J., Fall R., Goldan P., Guenther A. B., Hewitt C. N., Lamb B., Liu S., Trainer M., Westberg H. and Zimmerman P. (1992) Emissions of volatile organic compounds from vegetation and the implications for atmospheric chemistry. Global Biogeochem. Cycles 6, 389-430.
11. Finlayson-Pitts B. J. and Pitts J. N. (1986) Atmospheric Chemistry: Fundamentals and Experimental Techniques, p. 506 ff. Wiley-Interscience, New York.
12. Fung K. and Wright B. (1990) Measurement of formaldehyde and acetaldehyde using 2,4-dinitrophenylhydrazine-impregnated cartridges during the carbonaceous species methods comparison study. Aerosol Sci. Technol. 12, 44-48.
13. Geiß H. and Volz-Thomas A. (eds.) (1993) Lokale und regionale Ozonproduktion: Chemie und Transport. In Berichte des Forschungszentrums Jülich; No. 2764, Forschungszentrum Jülich GmbH, Zentralbibliothek, D-52425 Jülich.
14. Graedel T.-E. (1978) Carbonyl compounds. In Chemical Compounds in the Atmosphere, pp. 158-209. Academic Press, New York.
15. Gregori M., Lanzerstorfer Ch., Oberlinninger H., Puxbaum H., Biebl P., Gläser O. and Villinger J. (1989) Tauerntunnel -Luftschadstoffuntersuchung 1988. Bericht 4/89, Abteilung für Umweltanalytik, Institut für Analytische Chemie, Technische Universität Wien.
16. Grosjean D., Swanson R. D. and Ellis C. (1983) Carbonyls in Los Angeles air: contributions of direct emissions and photochemistry. Sci. Total Envir. 29, 65-85.
17. Grosjean D. (1988) Aldehydes, carboxylic acids and inorganic nitrate during NSMCS. Atmospheric Environment 22, 1637-1648.
18. Isidorov V. A., Zenkevich I. G. and Ioffe B. V. (1985) Volatile organic compounds in the atmosphere of forests. Atmospheric Environment 19, 1-8.
19. Kimmerer T. W. and Kozlowski T. T. (1982) Ethylene, ethane, acetaldehyde, and ethanol production by plants under stress. Plant. Physiol. 69, 840-847.
20. x regimes. J. geophys. Res. 96, 20,721-20,733.
21. Klemp D., Flocke F., Kramp F., Pätz W., Volz-Thomas A. and Kley D. (1993) Indications for biogenic sources of light olefins in the vicinity of Schauinsland/Black Forest (TOR station No. 11), Joint Workshop CEC/BIATEX of EUROTRAC, Aveiro, Portugal. In Air Pollution Research Report 47 (edited by Slanina J., Angeletti G. and Beilke S.), ISBN 2-87263-095-3, pp. 271-281.
22. Kley D., Geiss H., Klemp D., Kramp F., Su Y. and Volz-Thomas A. (1993) The importance of hydrocarbon measurements. In Proc. EUROTRAC Symp. 92 (edited by Borrell P.M. et al.), pp. 70-79. SPB Academic Publishing bv, The Hague, The Netherlands.
23. 8 hydrocarbons between Freiburg and Schauinsland: Implications for the budgets of olefins. In Proc. EUROTRAC Symp. 94 (edited by Borrell P. et al), pp. 373-378. SPB Academic Publishing bv, The Hague, The Netherlands.
24. Kramp F., Kley D. and Volz-Thomas A. (1995) Die Rolle reaktiver Kohlenwasserstoffe bei der Photooxidantienbildung in ländlichen Gebieten: Ein Beitrag zur Bilanzierung der photochemischen Ozonproduktion, Berichte des Forschungszentrum Jülich, Jülich-3050.
25. Lazrus A. L., Fong K. L. and Lind J. A. (1988) Automated fluorometric determination of formaldehyde in air. Anal. Chem. 60, 1074-1078.
26. Li S.-M., Anlauf K. G., Wiebe H. A. and Bottenheim J. W. (1994) Estimating primary and secondary production of HCHO in eastern North America based on gas phase measurements and principal component analysis. Geophys. Res. Lett. 21, 669-672.
27. Liu S. C., Trainer M., Fehsenfeld F. C., Parrish D. D., Williams E. J., Fahey D. W., Hübler G. and Murphy P. C. (1987) Ozone production in the rural troposphere and the implications for regional and global ozone distributions. J. geophys. Res. 92, 4191-4207.
28. Lowe D. C. and Schmidt U. (1983) Formaldehyde (HCHO) measurements in the nonurban atmosphere. J. geophys. Res. 88, 10,844-10,858.
29. Lowe D. C., Schmidt U., Ehhalt D. H., Frischkorn C. G. B. and Nürnberg H. W. (1981) Determination of formaldehyde in clean air. Envir. Sci. Technol. 15, 819-820.
30. Organikum (1981) Organisch-chemisches Grundpraktikum, pp. 486-487. VEB Deutscher Verlag der Wissenschaften.
31. 2 by differential optical absorption in the near UV. J. geophys. Res. 85, 7453-7458.
32. Platt U., Rateike M., Junkermann W., Rudolph J. and Ehhalt D. H. (1988) New tropospheric OH measurements. J. geophys. Res. 93, 5159-5166.
33. 3 carbonyl compounds at two rural sites in Central Ontario. Atmospheric Environment 25A, 2001-2015.
34. Schubert B., Schmidt U. and Ehhalt D. H. (1988) Untersuchungen zum Nachweis und zur Chemie von Formaldehyd und Acetaldehyd in der unteren Troposphäre, Berichte der Forschungsanlage Jülien; Nr. 2257, Forschungsanlage Jülich GmbH, Zentralbibliothek, D-52425 Jülich.
35. Slemr J. (1991) Determination of volatile carbonyl compounds in clean air. Fresenius J. Anal. Chem. 340, 672-677.
36. Slemr J., Schulz S., Seemann S. and Kern M. (1993) Development of techniques for the determination of major carbonyl compounds in clean air. In Proc. EUROTRAC Symp. 92 (edited by Borrell P. et al.), pp. 170-172. SPB Academic Publishing bv, The Hague, The Netherlands.
37. Volz-Thomas A. (1994) TOR Station Schauinsland. In The TOR Network, EUROTRAC special publication, ISS (edited by Cvitas T. and Kley D.), pp. 81-94. Garmisch-Partenkirchen.
38. Volz-Thomas A., Kley D., Buers H. J., Flocke F., Garthe H. J., Geiß H., Gilge S., Heil T., Houben N., Klemp D., Kramp F., Loup H., Mihelcic D., Müsgen P., Pätz H. W., Smit H. G. J. and Su Y. (1991) Local and regional ozone production: chemistry and transport. In EUROTRAC Annual Report, Part 9, TOR.
39. Volz-Thomas A., Flocke F., Garthe H. J., Geiß H., Gilge S., Heil T., Kley D., Klemp D., Kramp F., Mihelcic D., Pätz H. W., Schulz M. and Su Y. (1993) Photo-oxidants and precursors at Schauinsland, Black Forest. In Proc. of EUROTRAC Symp. 92 (edited by Borrell P. et al.), pp. 98-103. SPB Academic Publishing bv, The Hague, The Netherlands.