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Volumn 273, Issue 5274, 1996, Pages 480-483

Low-frequency Raman scattering and the fast relaxation process in glycerol

Author keywords

[No Author keywords available]

Indexed keywords

GLASS; GLYCEROL; HYDROXYL GROUP;

EID: 0029843624     PISSN: 00368075     EISSN: None     Source Type: Journal    
DOI: 10.1126/science.273.5274.480     Document Type: Article
Times cited : (35)

References (34)
  • 1
    • 0009071257 scopus 로고    scopus 로고
    • See, for example, C. A. Angell, Science 267, 1924 (1995); F. H. Stillinger, ibid., p. 1935; B. Frick and D. Richter, ibid., p. 1939.
    • (1995) Science , vol.267 , pp. 1924
    • Angell, C.A.1
  • 2
    • 0009071257 scopus 로고    scopus 로고
    • See, for example, C. A. Angell, Science 267, 1924 (1995); F. H. Stillinger, ibid., p. 1935; B. Frick and D. Richter, ibid., p. 1939.
    • Science , pp. 1935
    • Stillinger, F.H.1
  • 3
    • 0009071257 scopus 로고    scopus 로고
    • See, for example, C. A. Angell, Science 267, 1924 (1995); F. H. Stillinger, ibid., p. 1935; B. Frick and D. Richter, ibid., p. 1939.
    • Science , pp. 1939
    • Frick, B.1    Richter, D.2
  • 4
    • 0000978126 scopus 로고
    • J. P. Hansen, D. Levesque, J. Zinn-Justin, Eds. North-Holland, Amsterdam
    • W. Götze, in Liquids, Freezing, and the Glass Transition, J. P. Hansen, D. Levesque, J. Zinn-Justin, Eds. (North-Holland, Amsterdam, 1991), p. 287.
    • (1991) Liquids, Freezing, and the Glass Transition , pp. 287
    • Götze, W.1
  • 5
    • 0001513360 scopus 로고
    • M. Krüger, M. Soltwisch, I. Petscherizin, D. Quitmann, J. Chem. Phys. 96, 7352 (1992); Z. Pan, D. O. Henderson, S. H. Morgan, ibid. 101, 1767 (1994); V. N. Novikov, E. Duval, A. Kisliuk, A. P. Sokolov, ibid. 102, 4691 (1995).
    • (1992) J. Chem. Phys. , vol.96 , pp. 7352
    • Krüger, M.1    Soltwisch, M.2    Petscherizin, I.3    Quitmann, D.4
  • 6
    • 0028493205 scopus 로고
    • M. Krüger, M. Soltwisch, I. Petscherizin, D. Quitmann, J. Chem. Phys. 96, 7352 (1992); Z. Pan, D. O. Henderson, S. H. Morgan, ibid. 101, 1767 (1994); V. N. Novikov, E. Duval, A. Kisliuk, A. P. Sokolov, ibid. 102, 4691 (1995).
    • (1994) J. Chem. Phys. , vol.101 , pp. 1767
    • Pan, Z.1    Henderson, D.O.2    Morgan, S.H.3
  • 7
    • 0000169941 scopus 로고
    • M. Krüger, M. Soltwisch, I. Petscherizin, D. Quitmann, J. Chem. Phys. 96, 7352 (1992); Z. Pan, D. O. Henderson, S. H. Morgan, ibid. 101, 1767 (1994); V. N. Novikov, E. Duval, A. Kisliuk, A. P. Sokolov, ibid. 102, 4691 (1995).
    • (1995) J. Chem. Phys. , vol.102 , pp. 4691
    • Novikov, V.N.1    Duval, E.2    Kisliuk, A.3    Sokolov, A.P.4
  • 11
    • 0001489740 scopus 로고
    • E. Rössler, A. P. Sokolov, A. Kisliuk, D. Quitmann, Phys. Rev. B 49, 14967 (1994); S. Kojima, ibid. 47, 2924 (1993).
    • (1993) Phys. Rev. B , vol.47 , pp. 2924
    • Kojima, S.1
  • 12
    • 3743138534 scopus 로고
    • J. Wuttke et al., Phys. Rev. Lett. 72, 3052 (1994); F. Fujara, W. Petry, R. M. Diehl, W. Schnauss, H. Sillescu, Europhys. Lett 14, 563 (1991).
    • (1994) Phys. Rev. Lett. , vol.72 , pp. 3052
    • Wuttke, J.1
  • 16
    • 0027127088 scopus 로고
    • N. Pugliano and R. J. Saykally, Science 257, 1937 (1992); M. Schütz, T. Bürgi, S. Leutwyler, H. B. Bügi, J. Chem. Phys. 99, 5228 (1993); S. S. Xantheas and T. H. Dunnin Jr., ibid. 98, 8037 (1993).
    • (1992) Science , vol.257 , pp. 1937
    • Pugliano, N.1    Saykally, R.J.2
  • 17
    • 36449000231 scopus 로고
    • N. Pugliano and R. J. Saykally, Science 257, 1937 (1992); M. Schütz, T. Bürgi, S. Leutwyler, H. B. Bügi, J. Chem. Phys. 99, 5228 (1993); S. S. Xantheas and T. H. Dunnin Jr., ibid. 98, 8037 (1993).
    • (1993) J. Chem. Phys. , vol.99 , pp. 5228
    • Schütz, M.1    Bürgi, T.2    Leutwyler, S.3    Bügi, H.B.4
  • 18
    • 36449007707 scopus 로고
    • N. Pugliano and R. J. Saykally, Science 257, 1937 (1992); M. Schütz, T. Bürgi, S. Leutwyler, H. B. Bügi, J. Chem. Phys. 99, 5228 (1993); S. S. Xantheas and T. H. Dunnin Jr., ibid. 98, 8037 (1993).
    • (1993) J. Chem. Phys. , vol.98 , pp. 8037
    • Xantheas, S.S.1    Dunnin Jr., T.H.2
  • 19
    • 0001472897 scopus 로고
    • F. Huisken and M. Stemmler, Chem, Phys. Lett. 144, 391 (1988); O. Mó, M. Yáñez, J. Elguero, J. Mol. Struct. (Theochem.) 314, 73 (1994).
    • (1988) Chem, Phys. Lett. , vol.144 , pp. 391
    • Huisken, F.1    Stemmler, M.2
  • 22
    • 9444233063 scopus 로고    scopus 로고
    • note
    • As the MRO in glycerol, much larger structures such as the cyclic tetramer and pentamer are also probable, but in this work we concentrated on the vibrational properties of the cyclic trimer. Even if such larger structures are present in real liquids, our general observations and conclusions should remain valid.
  • 25
    • 9444282916 scopus 로고    scopus 로고
    • note
    • 3 symmetry.
  • 26
    • 9444253796 scopus 로고    scopus 로고
    • note
    • -1 (10)]. This is not surprising because the number of intermolecular hydrogen bonds in the glycerol trimer is six, whereas that in the methanol trimer is three.
  • 31
    • 84935365569 scopus 로고
    • The structures and energies of molecular oligomers abstracted from their crystal structures are, in general, not expected to be optimum for the isolated oligomers [see, for example, D. E. Williams and Y. Xiao, Acta Crystallogr. A49, 1 (1993)].
    • (1993) Acta Crystallogr. , vol.A49 , pp. 1
    • Williams, D.E.1    Xiao, Y.2
  • 34
    • 9444247254 scopus 로고    scopus 로고
    • note
    • We thank the Supercomputer Laboratory, Institute for Chemical Research, Kyoto University, for providing the computer time and for permission to use the Cray Y-MP2E/264 supercomputer.


* 이 정보는 Elsevier사의 SCOPUS DB에서 KISTI가 분석하여 추출한 것입니다.