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10544242504
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note
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The occupation probability is calculated by systematically eliminating each vibrational frequency from the density of states giving the number of ways to configure the energy among the remaining oscillators given n quanta of energy in the mth vibrational mode. The enhanced transition probability for absorption from the n to the (n + 1) level is (n + 1) times as likely as the (n = O) to (n = 1) transition. Similarly the emission probability from the n to the (n - 1) level is enhanced by a factor of n above the (n = I) to (n = O) transition.
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23
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10544242875
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The direct count Beyer-Swinehart algorithm was used to determine the sum and density of states
-
The direct count Beyer-Swinehart algorithm was used to determine the sum and density of states.
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-
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26
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10544226507
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note
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-1 intervals is solved simultaneously to give the overall unimolecular dissociation rate constants.
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-
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28
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0001686153
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3. The single charge cross section was multiplied by 11. The resulting collision rate is approximately the same as that calculated using the collisional cross section measured for this ion by Covey, T.; Douglas, D. J. J. Am. Soc. Mass Spectrom. 1993, 4, 616-623.
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35
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0028951473
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36
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10544249359
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note
-
The interaction with arginine-54, as shown in Figure 5, may reduce free rotation in the transition state. This would not be the case if this interaction was via a protonated residue on the b ion. Whether this is an issue depends on the shape and position of the barrier for the charge separation process.
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37
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10544242874
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Submitted for publication
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