Rational Synthesis of Unidimensional Mixed Valence Solids. Structural, Spectral, and Electrical Studies of Charge Distribution and Transport in Partially Oxidized Nickel and Palladium Bisdiphenylglyoximates

Journal of the American Chemical Society

Volumn 101, Issue 11, 1979, Pages 2921-2936

  Cowie, Martin ^a   Gleizes, Alain ^a   Grynkewich, Gregory W ^a   Kalina, Davida Webster ^a   Scaringe, Raymond P ^a   Ibers, James A ^a   Marks, Tobin J ^a   McClure, Malcolm S ^a   Kannewurf, Carl R ^a   Ruby, Stanley L ^b   Teitelbaum, Robert C ^b  

^a NORTHWESTERN UNIVERSITY   (United States)

^b ARGONNE NATIONAL LABORATORY   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

ELECTRONS; ORGANIC COMPOUNDS - PHYSICAL CHEMISTRY; PALLADIUM COMPOUNDS - OXIDATION; SPECTROSCOPY; X-RAY ANALYSIS;

OXIDIZED NICKEL BISDIPHENYLGLYOXIMATE; OXIDIZED PALLADIUM BISDIPHENYLGLYOXIMATE;

NICKEL COMPOUNDS;

EID: 0018467277     PISSN: 00027863     EISSN: 15205126     Source Type: Journal    
DOI: 10.1021/ja00505a021     Document Type: Article

References (169)

1. Devreese, J. T.; Evrard, R. P.; van Doren, V. E. “Highly Conducting One-Dimensional Solids”, Plenum Press; New York, 1979.
2. Miller, J. S.; Epstein, A. J. Ann. N.Y. Acad. Sci., 1978, 313.
3. Keller, H. J., Ed. “Chemistry and Physics of One-Dimensional Metals”, Plenum Press: New York, 1977.
4. Miller, J. S.; Epstein, A. J. Prog. Inorg. Chem. 1976, 20, 1-151.
5. Keller, H. J., Ed. “Low Dimensional Cooperative Phenomena”, Plenum Press: New York, 1975.
6. Soos, Z. G.; Klein In “Molecular Associations”, Foster, R., Ed.; Academic Press: New York, 1975.
7. Masuda, K.; Silver, M. “Charge and Energy Transfer in Organic Semiconductors”, Plenum Press: New York, 1974.
8. Interrante, L. V. “Extended Interactions between Metal Ions in Transition Metal Complexes”, ACS Symposium Series, No. 5, American Chemical Society: Washington, D.C., 1974.
9. Zeller, H. R. Festkorperprobleme, 1973, 13, 31-58.
10. Bloch, A. N.; Cowan, D. O.; Bechgaard, K.; Pyle, R. E.; Banks, R. H. Phys. Rev. Lett. 1975, 34, 1561-1564.
11. Ashwell, G. J.; Eley, D. D.; Willis, M. R. Nature (London) 1976, 259, 201-202.
12. Isett, L. C.; Perez-Albuerne, E. A. Solid State Commun. 1977, 21, 433-435.
13. Bechgaard, K.; Jacobsen, C. S.; Anderson, N. H. Solid State Commun. 1978, 25, 875-879.
14. Garito, A. F.; Heeger, A. J. Acc. Chem. Res. 1974, 7, 232-240.
15. Haddon, R. C. Nature (London) 1975, 256, 394-396.
16. Soos, Z. G. Annu. Rev. Phys. Chem. 1974, 25, 121-153.
17. Pouget, J. P.; Khanna, S. K.; Denoyer, F.; Comes, R.; Garito, A. F.; Heeger, A. J. Phys. Rev. Lett. 1976, 37, 437-440.
18. Torrance, J. B.; Scott, B. A.; Kaufman, F. B. Solid State Commun. 1975, 17, 1369-1373.
19. Butler, M. A.; Wudl, F.; Soos, Z. G. Phys. Rev. B 1975, 12, 4708-4719.
20. LaPlaca, S. J.; Corfield, P. W. R.; Thomas, R.; Scott, B. A. Solid State Commun. 1975, 17, 635-638.
21. Coppens, P. Phys. Rev. Lett. 1975, 35, 98-100.
22. Torrance, J. B. Acc. Chem. Res., 1979, 12, 79-86.
23. Torrance, J. B. Ann. N. Y. Acad. Sci. 1978, 313, 210-232.
24. Reise, A. H., Jr.; Hagley, V. S.; Petersen, S. W. J. Am. Chem. Soc. 1977, 99, 4184-4186.
25. Gordon, J. G., II; Williams, R.; Hsu, C.-H.; Cuellar, E.; Samson, S.; Mann, K.; Gray, H. B.; Hadek, V.; Somoano, R. Ann. N. Y. Acad. Sci. 1978, 313, 580-593.
26. Marks, T. J. Ann. N.Y. Acad. Sci. 1978, 313, 594-616.
27. Brown, L. D.; Kalina, D. W.; McClure, M. S.; Ruby, S. L.; Schultz, S.; lbers, J. A.; Kannewurf, C. R.; Marks, T. J. J. Am. Chem. Soc., following paper in this issue.
28. Gleizes, A.; Marks, T. J.; lbers, J. A. J. Am. Chem. Soc. 1975, 97, 3545-3546.
29. Marks, T. J.; Gleizes, A.; Lbers, J. A. “Abstracts of Papers”, 170th National Meeting of the American Chemical Society, Chicago, III., Aug 1975.
30. American Chemical Society: Washington, D.C., 1975; INOR 54.
31. Petersen, J. L.; Schramm, C. S.; Stojakovic, D. R.; Hoffman, B. M.; Marks, T. J. J. Am. Chem. Soc. 1977, 99, 286-288.
32. Schramm, C. S.; Stojakovic, D. R.; Hoffman, B. M.; Marks, T. J. Science 1978, 200, 47-48.
33. Peterson, J. L.; Schramm, C. S.; Scaringe, R. P.; Stojakovic, D. R.; Hoffman, B. M.; lbers, J. A.; Marks, T. J., manuscript in preparation.
34. Popov, A. I. MTP Int. Rev. Sci.: Inorg. Chem., Ser. One 1972, 3.
35. Huheey, J. H.; “Inorganic Chemistry”, 2nd Ed., Harper and Row: New York, 1978, pp 666-669.
36. Marks, T. J.; Webster, D. F.; Ruby, S. L.; Schultz, S. J. Chem. Soc., Chem. Commun. 1976, 444-445.
37. Teitelbaum, R. C.; Ruby, S. L.; Marks, T. J. J. Am. Chem. Soc. 1978, 100, 3215-3217.
38. Kalina, D. W.; Stojakovic, D. R.; Teitelbaum, R. C.; Marks, T. J., manuscript in preparation.
39. Williams, D. E.; Wohlauer, G.; Rundle, R. E. J. Am. Chem. Soc. 1959, 81, 755-756.
40. Edelman, L. E. J. Am. Chem. Soc. 1950, 72, 5765-5766.
41. Underhill, A. E.; Watkins, D. M.; Pethig, R. Inorg. Nucl. Chem. Lett. 1973, 9, 1269-1273.
42. Miller, J. S.; Griffiths, C. H. J. Am. Chem. Soc. 1977, 99, 749-755.
43. Mehne, L. F.; Wayland, B. B. Inorg. Chem. 1975, 14, 881-885.
44. Keller, H. J.; Seibold, K. J. Am. Chem. Soc. 1971, 93, 1309-1310.
45. Foust, A. S.; Soderberg, R. J. Am. Chem. Soc. 1967, 89, 5507-5508.
46. Foster, R.; “Organic Charge-Transfer Complexes”, Academic Press: New York, 1969.
47. Mulliken, R. S.; Person, W. B. “Molecular Complexes”, Wiley-Interscience: New York, 1969.
48. Barefield, E. K.; Mocella, M. T. J. Am. Chem. Soc. 1975, 97, 4238-4246.
49. Lovecchio, F. V.; Gore, E. S.; Busch, D. H. J. Am. Chem. Soc. 1974, 96, 3109-3118.
50. Dolphin, D.; Niem, T.; Felton, R. H.; Fujita, I. J. Am. Chem. Soc. 1975, 97, 5288-5290.
51. Lappin, A. G.; Murray, C. K.; Margerum, D. W. Inorg. Chem. 1978, 17, 1630-1634.
52. Johnson, E. C.; Niem, T.; Dolphin, D. Can. J. Chem. 1978, 56, 1381-1388.
53. Cooper, C. B. Ph.D. Thesis, Northwestern University, July 1978.
54. Powell, M. J. D. Comput. J. 1965, 7, 303-307.
55. Ruby, S. L. “Mossbauer Effect Methodology”, Vol. 8; 1973; pp 263-276.
56. Schafer, D. E.; Wudl, F.; Thomas, G. A.; Ferraris, J. P.; Cowan, D. D. Solid State Commun. 1974, 14, 347-351.
57. Cowie, M.; lbers, J. A. Inorg. Chem. 1976, 15, 552-557.
58. Doedens, R. J.; lbers, J. A. Inorg. Chem. 1967, 6, 204-210.
59. Lenhert, P. G. J. Appl. Crystallogr. 1975, 8, 568-570.
60. D. T.; Waber, J. T. “International Tables for X-ray Crystallography”, Vol. IV; Kynoch Press: Birmingham, England, 1974.
61. R. F.; Davidson, E. R.; Simpson, W. T. J. Chem. Phys. 1965, 42, 3175-3187.
62. Cromer, D. T.; Liberman, D. J. Chem. Phys. 1970, 53, 1891-1898.
63. Warren, B. E. “X-ray Diffraction”, Addison-Wesley: Reading, Mass., 1969; p 35.
64. Endres, H.; Keller, H. J.; Megnamisi-Belombe, M.; Moroni, W.; Pritzkow, H.; Weiss, J.; Comes, R. Acta Crystallogr, Sect. A 1976, 32, 954-957.
65. Smith, D. L.; Luss, H. R. Acfa Crystallogr., Sect. B 1977, 33, 1744-1749.
66. Huml, K. Acta Crystallogr 1967, 22, 29-32.
67. Beyeler, H. U. Phys. Rev. Lett. 1976, 37, 1557-1560.
68. Herbstein, F. H.; Kapon, M. Acfa Crystallogr., Sect. A 1972, 28, S74.
69. Endres, H.; Keller, H. J.; Moroni, W.; Weiss, J. Acta Crystallogr, Sect. B 1975, 31, 2357-2358.
70. Robertson, J. M.; Woodward, I. J. Chem. Soc. 1937, 219-220.
71. Millar, M.; Holm. R. H. J. Am. Chem. Soc. 1975, 97, 6052-6058.
72. Peng, S.-M.; Ibers, J. A.; Millar, M.; Holm, R. H. J. Am. Chem. Soc. 1976, 98, 8037-8041.
73. Peng, S.-M.; Goedken, V. L. J. Am. Chem. Soc. 1976, 98, 8500-8510.
74. Charlson, A. J.; Stephens, F. S.; Vagg, R. S.; Watton, E. C. Inorg. Chim. Acta 1977, 25, L51-L52.
75. “Handbook of Chemistry and Physics”, 57th ed.; Chemical Rubber Publishing Co.: Cleveland, Ohio, 1976-1977; p F-216.
76. Shannon, R. D. Acta Crystallogr, Sect. A 1976, 32, 751-767.
77. Sacconi, L. Transition Met. Chem. 1968, 4, 199-298.
78. Fleischer, E. B. J. Am. Chem. Soc. 1963, 85, 146-148.
79. Hamor, T. A.; Caughey, W. S.; Hoard, J. L. J. Am. Chem. Soc. 1965, 87, 2305-2312.
80. Meyer, E. F., Jr. Acta Crystallogr, Sect. B 1972, 28, 2162-2167.
81. Cullen, D. L.; Meyer, E. F., Jr. J. Am. Chem. Soc. 1974, 96, 2095-2102.
82. Dwyer, P. N.; Buchler, J. W.; Scheidt, W. R. J. Am. Chem. Soc. 1974, 96, 2789-2795.
83. Guinier, A. “X-ray Diffraction in Crystals, Imperfect Crystals, and Amorphous Bodies”, W.H. Freeman: San Francisco, 1963; p 154.
84. Johnson, B. B.; Peticolas, W. L. Annu. Rev. Phys. Chem. 1976, 27, 465-491.
85. Warshel, A. Annu. Rev. Biophys. Bioeng. 1977, 6, 273-300.
86. Spiro, T. G. “Chemical and Biochemical Applications of Lasers”, Moore, C. B., Ed.; Academic Press: New York, 1974.
87. Tang, J.; Albrecht, A. C. “Raman Spectroscopy”, Vol. 2; Szymanski, H. A., Ed.; Plenum Press: New York, 1970.
88. Johnson, B. B.; Nafie, L. A.; Peticholas, W. L. Chem. Phys. 1977, 19, 303-311.
89. Nafie, L. A.; Pastor, R. W.; Dobrowiak, J. C.; Woodruff, W. H. J. Am. Chem. Soc. 1976, 98, 8007-8014.
90. Stein, P.: Miskowski, V.; Woodruff, W. H.; Griffin, J. P.; Werner, K. G.; Gaber, B. P.; Spiro, T. G. J. Chem. Phys. 1976, 64, 2159-2167.
91. Mingardi, M.; Siebrand, W. J. Chem. Phys. 1975, 62, 1074-1085.
92. Kiefer, W. Appl. Spectrosc. 1974, 28, 115-133.
93. Runsink, J.; Swen-Walstra, S.; Migchelsen, T. Acta. Crystallogr., Sect. B 1972, 28, 1331-1335.
94. Maki, A. G.; Forneris, R. Spectrochim. Acta, Part A 1967, 23, 867-880.
95. Haywood, G. C.; Hendra, P. J. Spectrochim. Acta, Part A, 1967, 23, 2309-2314.
96. Gabes, W.; Nijman-Meester, M.A.M. Inorg. Chem. 1973, 12, 589-592.
97. Datta, S. N.; Ewig, C. S.; Van Wazer, J. R. J. Mol. Struct. 1978, 48, 407-416.
98. Reddy, J. M.; Knox, K.; Robin, M. B. J. Chem. Phys. 1964, 40, 1082-1089.
99. P. Cougrand, A.; Flandrois, S.; Chasseau, D.; Gaultier, J.; Hauw, C.; Dupuis, P. Led. Notes Phys. 1977, 65, 493-498.
100. Brown, R. D.; Nunn, E. K. Aus. J. Chem. 1966, 19, 1567-1576.
101. Migchelsen, T.; Vos, A. Acta Crystallogr 1967, 22, 812-815.
102. Rundle, R. E. Acta Crystallogr. 1961, 14, 585-589.
103. Anderson, A.; Sun, R. S. Chem. Phys. Lett. 1970, 6, 611-616.
104. Havinga, E. E.; Boswijk, K. H.; Wiebenga, E. H. Acta Crystallogr. 1954, 7, 487-490.
105. Herbstein, F. H.; Kapon, M. Nature (London) 1972, 239, 153-154.
106. Havinga, E. E.; Wiebenga, E. H. Acta Crystallogr 1958, 11, 733-737.
107. Hach, R. J.; Rundle, R. E. J. Am. Chem. Soc. 1951, 73, 4321-4324.
108. Gabes, W.; Stufkens, D. J. Spectrochim. Acta, Part A 1974, 30, 1835-1841.
109. Robin, M. B. J. Chem. Phys. 1964, 40, 3369-3377.
110. Kalina, D. W.; McClure, M. S.; Kannewurf, C. R.; Marks, T. J., manuscript in preparation.
111. Kamaras, K.; Mihaly, G.; Griiner, G.; Janossy, A. J. Chem. Soc., Chem. Commun. 1978, 974-975.
112. Sunder, S.; Mendelsohn, R.; Bernstein, H. J. J. Chem. Phys. 1975, 63, 573-580.
113. Friedman, J. M.; Hochstrasser, R. M. J. Am. Chem. Soc. 1976, 98, 4043-4048.
114. Shelnutt, J. A.; O'Shea, D. C.; Yu, N.-T.; Cheung, L. D.; Felton, R. H. J. Chem. Phys. 1976, 64, 1156-1165.
115. Woodruff, W. M.; Pastor, R. W.; Dobrowiak, J. C. J. Am. Chem. Soc. 1976, 98, 7999-8006.
116. Gibb, T. C. “Principles of Mossbuaer Spectroscopy”, Chapman and Hall: London, 1976.
117. Bancroft, G. M.; Platt, R. H. Adv. Inorg. Chem. Radiochem. 1972, 15, 59-258.
118. Potasek, M. J.; Debrunner, P. G.; Morrison, W. H., Jr.; Hendrickson, D. N. J. Chem. Phys. 1974, 60, 2203-2206.
119. Ehrlich, B. S.; Kaplan, M. J. Chem. Phys. 1969, 51, 603-606.
120. Lucken, E. A. C. “Nuclear Quadrupole Coupling Constants”, Academic Press: New York, 1969.
121. Dailey, B. P.; Townes, C. H. J. Chem. Phys. 1955, 23, 118-123.
122. Ruby, S. L.; Shenoy, G. K. “Mossbauer Isomer Shifts”, Shenoy, G. K.; Wagner, F. E., Eds., North-Holland Publishing Co.: Amsterdam, 1978.
123. Bukshpan, S.; Goldstein, C.; Sonnino, T.; May, L.; Pasternak, M. J. Chem. Phys. 1975, 62, 2606-2609.
124. deWaard, H. “MOssbauer Effect Data Index”, 1973; pp 447-494.
125. Anex, B. G. ACS Symposium Series, No. 5, American Chemical Society; Washington, D.C., 1974; pp 276-300.
126. Hara, Y.; Shirotani, I.; Onodera, A. Solid State Commun. 1976, 19, 171-175.
127. Ohashi, Y.; Hanazaki, I.; Nagakura, S. Inorg. Chem. 1970, 9, 2551-2556.
128. Anex, B. G.; Krist, F. K. J. Am. Chem. Soc. 1967, 89, 6114-6125.
129. Banks, C. V.; Barnum, D. W. J. Am. Chem. Soc. 1958, 80, 4767-4772.
130. Basu, G.; Cook, G. M.; Belford, R. L. Inorg. Chem. 1964, 3, 1361-1368.
131. Zahner, J. C.; Drickamer, H. G. J. Chem. Phys. 1960, 33, 625-1628.
132. Beattie, J. K.; Hush, N. S.; Taylor, P. R. Inorg. Chem. 1976, 15, 992-993.
133. Hush, N. S. Prog. Inorg. Chem, 1967, 8, 391-444.
134. Robin, M. B.; Day, P. Adv. Inorg. Chem. Radiochem. 1967, 10, 247-422.
135. Stojakovic, D. R. Ph.D. Thesis, Northwestern University, Evanston, III., Aug 1977.
136. Swingle, R. S., II; Riggs, W. M. Crit. Rev. Anal. Chem. 1975, 5, 267-321.
137. Jolly, W. L. Top. Curr. Chem. 1977, 71, 149-182.
138. Coord. Chem. Rev. 1974, 13, 47-81.
139. Hercules, D. M.; Carver, J. C., Anal. Chem. 1974, 46, 133R-150R.
140. Cowan, D. O.; Park, J.; Barber, M.; Swift, P. Chem. Commun. 1971, 1444-1446.
141. Cahen, D.; Lester, J. E. Chem. Phys. Lett. 1973, 18, 108-111.
142. Burroughs, P.; Hammett, A.; Orchard, A. F. J. Chem. Soc. Dalton Trans., 1974, 565-567.
143. Thomas, J. M.; Tricker, M. J. J. Chem. Soc., Faraday Trans. 2 1975, 329-336.
144. Helmer, J. E. J. Electron Spectrosc. Relat. Phenom. 1973, 1, 259-267.
145. Oku, M.; Hirokawa, K. J. Electron. Spectrosc. Relat. Phenom. 1976, 8, 475-481.
146. Orchard, A. F.; Thornton, G. J. Chem. Soc., Dalton Trans. 1977, 1238-1240.
147. Hush, N. S. Chem. Phys. 1975, 10, 361-366.
148. Matienzo, L. J.; Yin, L. I.; Grim, S. O.; Swartz, W. D. Inorg. Chem. 1973, 12, 2762-2769.
149. Kumar, G.; Blackburn, J. R.; Albridge, R. G.; Moddeman, W. E.; Jones, M. M. Inorg. Chem. 1972, 11, 296-300.
150. Clark, D. T.; Adams, D. B. Chem. Commun. 1971, 602-604.
151. Hedman, Jr.; Klasson, M.; Nilsson, R.; Nordling, C.; Sorokina, M. F.; Kljushnikov, O. I.; Nemnonov, S. A.; Trapenznikov, V. A.; Zyryanov, V. G. Phys. Scr. 1971, 4, 195-201.
152. Lin, L. I.; Ghose, S.; Alder, I. Appl. Spectrosc. 1972, 26, 355-357.
153. Kim, K. S.; Baitinger, W. E.; Amy, J. W.; Winograd, N. J. J. Electron Spectrosc. Relat. Phenom. 1974, 5, 351-357.
154. Riggleman, B. M.; Drickamer, H. G. J. Chem. Phys. 1963, 38, 2721-2724.
155. Jacobsen, C. S.; Mortensen, K.; Andersen, J. R.; Bechgaard, K. Phys. Rev. B 1978, 18, 905-921.
156. Wheland, R. C.; Gillson, J. L. J. Am. Chem. Soc. 1976, 98, 3916-3925.
157. Chiang, C. K.; Druy, M. A.; Gau, S. C.; Heeger, A. J.; Louis, E. J.; MacDiarmid, A. G.; Park, Y. W.; Shirakawa, H. J. Am. Chem. Soc. 1978, 100, 1013-1015.
158. Berlinsky, A. J. Contemp. Phys. 1976, 17, 331-354.
159. Thomas, G. A., et al. Phys. Rev. B 1976, 13, 5105-5110.
160. Bloch, A. N.; Welsman, R. B.; Varma, C. M. Phys. Rev. Lett. 1972, 28, 753-756.
161. Shchegolev, I. F. Phys. Status Solidi A 1972, 12, 9-45.
162. Shante, V. K. S. Phys. Rev. B 1977, 16, 2597-2612.
163. Cohen, M. H. Led. Notes Phys. 1977, 65, 225-265.
164. Mihaly, G.; Ritvay-Emandity, K.; Janossy, A.; Holczer, K.; Griiner, G. Solid State Commun. 1977, 21, 721-724.
165. Mott, N. F. “Metal-Insulator Transitions”, Taylor and Francis: London, 1974.
166. Epstein, A. J.; Conwell, E. M.; Sandman, D. J.; Miller, J. S. Solid State Commun. 1977, 23, 335-358.
167. Epstein, A. J.; Conwell, E. M. Solid State Commun. 1977, 24, 627-630.
168. Conwell, E. M. Phys. Rev. Lett. 1977, 39, 777-780.
169. Williams, J. M.; Petersen, J. L.; Gerdes, H. M.; Peterson, S. W. Phys. Rev. Lett. 1974, 33, 1079-1081.