Proton transfer dynamics in the first excited singlet state of malonaldehyde

Journal of Chemical Physics

Volumn 107, Issue 14, 1997, Pages 5617-5620

  Arias, Angela A ^a   Wasserman, Thierry A W ^a   Vaccaro, Patrick H ^a  

^a YALE UNIVERSITY   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

EID: 0012113590     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.474263     Document Type: Article

References (51)

1. P. Löwdin, Rev. Mod. Phys. 35. 724 (1963); D. Devault, Q. Rev. Biophys. 13, 387 (1980); F. Hibbert, Adv. Phys. Org. Chem. 22, 113 (1986).
2. P. Löwdin, Rev. Mod. Phys. 35. 724 (1963); D. Devault, Q. Rev. Biophys. 13, 387 (1980); F. Hibbert, Adv. Phys. Org. Chem. 22, 113 (1986).
3. P. Löwdin, Rev. Mod. Phys. 35. 724 (1963); D. Devault, Q. Rev. Biophys. 13, 387 (1980); F. Hibbert, Adv. Phys. Org. Chem. 22, 113 (1986).
4. W. F. Rowe, R. W. Duerst, and E. B. Wilson, J. Am. Chem. Soc. 98, 4021 (1976); P. Turner et al., ibid. 106, 2265 (1984).
5. W. F. Rowe, R. W. Duerst, and E. B. Wilson, J. Am. Chem. Soc. 98, 4021 (1976); P. Turner et al., ibid. 106, 2265 (1984).
6. S. L Baughcum et al., J. Am. Chem. Soc. 103, 6296 (1981); Z. Smith, E. B. Wilson, and R. W. Duerst, Spectrochim. Acta. A 39, 1117 (1983); S. L. Baughcum et al. J. Am. Chem. Soc. 106, 2260 (1984).
7. S. L Baughcum et al., J. Am. Chem. Soc. 103, 6296 (1981); Z. Smith, E. B. Wilson, and R. W. Duerst, Spectrochim. Acta. A 39, 1117 (1983); S. L. Baughcum et al. J. Am. Chem. Soc. 106, 2260 (1984).
8. S. L Baughcum et al., J. Am. Chem. Soc. 103, 6296 (1981); Z. Smith, E. B. Wilson, and R. W. Duerst, Spectrochim. Acta. A 39, 1117 (1983); S. L. Baughcum et al. J. Am. Chem. Soc. 106, 2260 (1984).
9. M J. Frisch et al., J. Chem. Phys. 82, 4194 (1985).
10. D. W. Firth et al., J. Chem. Phys. 94, 1812 (1991).
11. 2v) transition state.
12. P. R. Bunker, Molecular Symmetry and Spectroscopy (Academic, New York, 1979).
13. N. Shida, P. F. Barbara, and J. E. Almlöf, J. Chem. Phys. 91, 4061 (1989).
14. P. F. Barbara, P. K. Walsh, and L. E. Brus, J. Phys. Chem. 93, 29 (1989).
15. H. Ozeki et al., J. Chem. Phys. 99, 56 (1993).
16. C. J. Seliskar and R. E. Hoffman, Chem. Phys. Lett. 43, 481 (1976).
17. C. J. Seliskar and R. E. Hoffman, J. Am. Chem. Soc. 99, 7072 (1977); J. Mol. Spectrosc. 88, 30 (1981).
18. C. J. Seliskar and R. E. Hoffman, J. Am. Chem. Soc. 99, 7072 (1977); J. Mol. Spectrosc. 88, 30 (1981).
19. D. W. Firth, P. F. Barbara, and H. P. Trommsdorff, Chem. Phys. 136, 349 (1989).
20. K. Luth and S. Scheiner, J. Phys. Chem. 98, 3582 (1994).
21. Q. Zhang et al., J. Chem. Phys. 96, 1640 (1992); S. A. Kandel et al., Proc. SPIE 1858, 126 (1993); T. A. W. Wasserman et al., ibid. 2548, 220 (1995); Chem. Phys. Lett. 262, 329 (1996); T. A. W. Wasserman, P. H. Vaccaro, and B. R. Johnson, J. Chem. Phys. 106, 6314 (1997).
22. Q. Zhang et al., J. Chem. Phys. 96, 1640 (1992); S. A. Kandel et al., Proc. SPIE 1858, 126 (1993); T. A. W. Wasserman et al., ibid. 2548, 220 (1995); Chem. Phys. Lett. 262, 329 (1996); T. A. W. Wasserman, P. H. Vaccaro, and B. R. Johnson, J. Chem. Phys. 106, 6314 (1997).
23. Q. Zhang et al., J. Chem. Phys. 96, 1640 (1992); S. A. Kandel et al., Proc. SPIE 1858, 126 (1993); T. A. W. Wasserman et al., ibid. 2548, 220 (1995); Chem. Phys. Lett. 262, 329 (1996); T. A. W. Wasserman, P. H. Vaccaro, and B. R. Johnson, J. Chem. Phys. 106, 6314 (1997).
24. Q. Zhang et al., J. Chem. Phys. 96, 1640 (1992); S. A. Kandel et al., Proc. SPIE 1858, 126 (1993); T. A. W. Wasserman et al., ibid. 2548, 220 (1995); Chem. Phys. Lett. 262, 329 (1996); T. A. W. Wasserman, P. H. Vaccaro, and B. R. Johnson, J. Chem. Phys. 106, 6314 (1997).
25. Q. Zhang et al., J. Chem. Phys. 96, 1640 (1992); S. A. Kandel et al., Proc. SPIE 1858, 126 (1993); T. A. W. Wasserman et al., ibid. 2548, 220 (1995); Chem. Phys. Lett. 262, 329 (1996); T. A. W. Wasserman, P. H. Vaccaro, and B. R. Johnson, J. Chem. Phys. 106, 6314 (1997).
26. P. H. Vaccaro, in Molecular Dynamics and Spectroscopy by Stimulated Emission Pumping, edited by H. L. Dai and R. W. Field (World Scientific, Singapore, 1995), Chap. 1.
27. P. H. Vaccaro, in Nonlinear Spectroscopy for Molecular Structure Determination, edited by E. Hirota, R. W. Field, J. P. Maier, and S. Tsuchiya (Blackwell, London, 1997).
28. R. L. Farrow and D. J. Rakestraw, Science 257, 1894 (1992).
29. T. J. Butenhoff and E. A. Rohlfing, J. Chem. Phys. 97, 1595 (1992); ibid. 98, 5460, 5469 (1993); J. R. Dunlop and E. A. Rohlfing, ibid. 100, 856 (1993), J. D. Tobiason, J. R. Dunlop, and E. A. Rohlfing, ibid. 97, 1448 (1995).
30. T. J. Butenhoff and E. A. Rohlfing, J. Chem. Phys. 97, 1595 (1992); ibid. 98, 5460, 5469 (1993); J. R. Dunlop and E. A. Rohlfing, ibid. 100, 856 (1993), J. D. Tobiason, J. R. Dunlop, and E. A. Rohlfing, ibid. 97, 1448 (1995).
31. T. J. Butenhoff and E. A. Rohlfing, J. Chem. Phys. 97, 1595 (1992); ibid. 98, 5460, 5469 (1993); J. R. Dunlop and E. A. Rohlfing, ibid. 100, 856 (1993), J. D. Tobiason, J. R. Dunlop, and E. A. Rohlfing, ibid. 97, 1448 (1995).
32. T. J. Butenhoff and E. A. Rohlfing, J. Chem. Phys. 97, 1595 (1992); ibid. 98, 5460, 5469 (1993); J. R. Dunlop and E. A. Rohlfing, ibid. 100, 856 (1993), J. D. Tobiason, J. R. Dunlop, and E. A. Rohlfing, ibid. 97, 1448 (1995).
33. E. F. McCormack et al., Chem. Phys. Lett. 211, 147 (1993); 227, 656 (1994); E. F. McCormack et al., J. Chem. Phys. 102, 4740 (1995).
34. E. F. McCormack et al., Chem. Phys. Lett. 211, 147 (1993); 227, 656 (1994); E. F. McCormack et al., J. Chem. Phys. 102, 4740 (1995).
35. E. F. McCormack et al., Chem. Phys. Lett. 211, 147 (1993); 227, 656 (1994); E. F. McCormack et al., J. Chem. Phys. 102, 4740 (1995).
36. R. L. Abrams et al., in Optical Phase Conjugation, edited by R. A. Fisher (Academic, San Diego, 1983), p. 211.
37. S. Mukamel, Principles of Nonlinear Optical Spectroscopy (Oxford University Press, New York. 1995).
38. R. L. Vander Wal, R. L. Farrow, and D. J. Rakestraw, High-Resolution Investigation of Degenerate Four-Wave Mixing in the γ(0,0) Band of Nitric Oxide, 24th (International) Symposium on Combustion, 1992, p. 1653; E. J. Friedman-Hill, L. A. Rahn, and R. L. Farrow, J. Chem. Phys. 100, 4065 (1994).
39. R. L. Vander Wal, R. L. Farrow, and D. J. Rakestraw, High-Resolution Investigation of Degenerate Four-Wave Mixing in the γ(0,0) Band of Nitric Oxide, 24th (International) Symposium on Combustion, 1992, p. 1653; E. J. Friedman-Hill, L. A. Rahn, and R. L. Farrow, J. Chem. Phys. 100, 4065 (1994).
40. S. Williams, R. N. Zare, and L. A. Rahn, J. Chem. Phys. 101, 1072, 1093 (1994).
41. R. Hüttel, Chem. Ber. 74, 1825 (1941); E. J. J. Grabowski and R. L. Autrey, Tetrahedron 25, 4315 (1969).
42. R. Hüttel, Chem. Ber. 74, 1825 (1941); E. J. J. Grabowski and R. L. Autrey, Tetrahedron 25, 4315 (1969).
43. 1 malonaldehyde is probably much longer than the 10 ps lower limit established by measured spectral linewidths.
44. R. L. Farrow, T. Dreier, and D. J. Rakestraw, J. Opt. Soc. Am. B 9, 1770 (1992).
45. T. Azumi and K. Matsnzaki, Photochem. Photobiol. 25, 315 (1977); I. Özkan and L. Goodman, Chem. Rev. 79, 275 (1979); G. Fisher, Vibronic Coupling: The Interaction Between the Electronic and Nuclear Motions (Academic, London, 1984).
46. T. Azumi and K. Matsnzaki, Photochem. Photobiol. 25, 315 (1977); I. Özkan and L. Goodman, Chem. Rev. 79, 275 (1979); G. Fisher, Vibronic Coupling: The Interaction Between the Electronic and Nuclear Motions (Academic, London, 1984).
47. T. Azumi and K. Matsnzaki, Photochem. Photobiol. 25, 315 (1977); I. Özkan and L. Goodman, Chem. Rev. 79, 275 (1979); G. Fisher, Vibronic Coupling: The Interaction Between the Electronic and Nuclear Motions (Academic, London, 1984).
48. J. A. Pople and J. W. Sidman, J. Chem. Phys. 26, 1270 (1957); J. R. Henderson, ibid. 44, 3496 (1966); S. H. Lin, Proc. R. Soc. London, Ser. A 352, 57 (1976); K. K. Innes, J. Mol. Spectrosc. 99, 294 (1983).
49. J. A. Pople and J. W. Sidman, J. Chem. Phys. 26, 1270 (1957); J. R. Henderson, ibid. 44, 3496 (1966); S. H. Lin, Proc. R. Soc. London, Ser. A 352, 57 (1976); K. K. Innes, J. Mol. Spectrosc. 99, 294 (1983).
50. J. A. Pople and J. W. Sidman, J. Chem. Phys. 26, 1270 (1957); J. R. Henderson, ibid. 44, 3496 (1966); S. H. Lin, Proc. R. Soc. London, Ser. A 352, 57 (1976); K. K. Innes, J. Mol. Spectrosc. 99, 294 (1983).
51. J. A. Pople and J. W. Sidman, J. Chem. Phys. 26, 1270 (1957); J. R. Henderson, ibid. 44, 3496 (1966); S. H. Lin, Proc. R. Soc. London, Ser. A 352, 57 (1976); K. K. Innes, J. Mol. Spectrosc. 99, 294 (1983).