Time-resolved photoelectron angular distributions: A nonperturbative theory

Journal of Chemical Physics

Volumn 107, Issue 19, 1997, Pages 7859-7868

  Seideman, Tamar ^a,b  

^a HARVARD UNIVERSITY   (United States)

^b NATIONAL RESEARCH COUNCIL CANADA   (Canada)

Author keywords

[No Author keywords available]

Indexed keywords

EID: 0001657715     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.475098     Document Type: Article

References (64)

1. For reviews see (a) A. H. Zewail, in Femtosecond Chemistry, edited by J. Manz and L. Wöste (Weinheim, Basel, 1995), p. 15; (b) A. H. Zewail, Femtochemistry: Ultrafast Dynamics of the Chemical Bond (World Scientific, Singapore, 1994).
2. For reviews see (a) A. H. Zewail, in Femtosecond Chemistry, edited by J. Manz and L. Wöste (Weinheim, Basel, 1995), p. 15; (b) A. H. Zewail, Femtochemistry: Ultrafast Dynamics of the Chemical Bond (World Scientific, Singapore, 1994).
3. (a) A. Zavriyev, I. Fischer, D. M. Villeneuve, and A. Stolow, Chem. Phys. Lett. 234, 281 (1995);
4. (b) I. Fischer, D. M. Villeneuve, M. J. J. Vrakking, and A. Stolow, J. Chem. Phys. 102, 5566 (1995);
5. (c) M. J. J. Vrakking, I. Fischer, D. M. Villeneuve, and A. Stolow, J. Chem. Phys. 103, 4538 (1995);
6. (d) M. J. J. Vrakking, D. M. Villeneuve, and A. Stolow, J. Chem. Phys. 105, 5647 (1996);
7. (e) M. J. J. Vrakking, D. M. Villeneuve, and A. Stolow, Phys. Rev. A 54, 37R (1996).
8. (a) T. Baumert, V. Engel, C. Meier, and G. Gerber, Chem. Phys. Lett. 200, 488 (1992);
9. (b) T. Baumert, R. Thalweiser, V. Weiss, and G. Gerber, in Femtosecond Chemistry, edited by J. Manz and L. Wöste (Weinheim, Basel, 1995), p. 397 and references therein;
10. (c) T. Baumert, R. Thalweiser, V. Weiss, and G. Gerber, in Advances in Chemical Physics-Photochemistry: Chemical Reactions and their Control on the Femtosecond Time Scale, edited by I. Prigogine and S. Rice (Wiley, New York, in press);
11. (d) A. Assion, T. Baumert, J. Helbing, V. Seyfried, and G. Gerber, Phys. Rev. A 55, 1899 (1997).
12. M. Blackwell, P. Ludowise, and Y. Chen, J. Chem. Phys. 107, 283 (1997).
13. Femtosecond negative ion-neural-positive ion spectroscopy is described in S. Wolf, G. Sommerer, S. Rutz, E. Schreiber, T. Leisner, L. Woste, and R. S. Berry, Phys. Rev. Lett. 74, 4177 (1995). D. W. Boo, Y. Ozaki, L. H. Andersen, and W. C. Lineberger, J. Chem. Phys. (in press), and references therein.
14. Femtosecond negative ion-neural-positive ion spectroscopy is described in S. Wolf, G. Sommerer, S. Rutz, E. Schreiber, T. Leisner, L. Woste, and R. S. Berry, Phys. Rev. Lett. 74, 4177 (1995). D. W. Boo, Y. Ozaki, L. H. Andersen, and W. C. Lineberger, J. Chem. Phys. (in press), and references therein.
15. (a) J. M. Papanikolas, R. M. Williams, P. D. Kleiber, J. L. Hart, C. Brink, and S. R. Leone, J. Chem. Phys. 103, 7269 (1995);
16. (b) R. M. Williams, J. M. Papanikolas, J. Rathje and S. R. Leone, J. Chem. Phys. 106, 8299 (1997);
17. (c) J. M. Papanikolas, R. M. Williams, and S. R. Leone, J. Chem. Phys. (in press).
18. B. J. Greenblatt, M. T. Zanni, and D. M. Neumark, Chem. Phys. Lett. 258, 523 (1996); Science (in press).
19. B. J. Greenblatt, M. T. Zanni, and D. M. Neumark, Chem. Phys. Lett. 258, 523 (1996); Science (in press).
20. See, for instance, Y. S. Lee, in Femtosecond Chemistry, edited by J. Manz and L. Wöste (Weinheim, Basel, 1995), p. 273.
21. See, for instance, (a) J. Cao and K. R. Wilson, J. Chem. Phys. 106, 5062 (1997);
22. (b) S. Yu. Grebenshchikov, C. Beck, H. Flöthmann, D. H. Mordaut, and R. Schinke, Chem. Phys. Lett. 271, 197 (1997).
23. M. Seel and W. Domcke, J. Chem. Phys. 95, 7806 (1991).
24. (a) C. Meier and V. Engel, J. Chem. Phys. 101, 2673 (1994);
25. (b) M. Braun, C. Meier and V. Engel, J. Chem. Phys. 103, 7907 (1995);
26. (c) M. Braun, C. Meier and V. Engel, J. Chem. Phys. 105, 530 (1996).
27. See, for instance, (a) S. W. Allendorf, D. J. Leahy, D. C. Jacobs, and R. N. Zare, J. Chem. Phys. 91, 2216 (1989);
28. (b) K. L. Reid, D. J. Leahy, and R. N. Zare, J. Chem. Phys. 95, 1746 (1991);
29. (c) D. J. Leahy, K. L. Reid, H. Park and R. N. Zare, J. Chem. Phys. 97, 4948 (1992);
30. (d) H. Park and R. N. Zare, J. Chem. Phys. 106, 2239 (1997), and references therein to related work by the same group.
31. See, for instance, (a) S. N. Dixit and V. McKoy, J. Chem. Phys. 82, 3546 (1985); (b) S. N. Dixit, D. L. Lynch, and V. McKoy, Phys. Rev. A 32, 1267 (1985); (c) S. N. Dixit and V. McKoy, Chem. Phys. Lett. 128, 49 (1986); (d) R. L. Dubs, V. McKoy and S. N. Dixit, J. Chem. Phys. 88, 968 (1988); (e) H. Rudolph and V. McKoy, J. Chem. Phys. 91, 2235 (1989), and references therein to related work by the same group.
32. See, for instance, (a) S. N. Dixit and V. McKoy, J. Chem. Phys. 82, 3546 (1985); (b) S. N. Dixit, D. L. Lynch, and V. McKoy, Phys. Rev. A 32, 1267 (1985); (c) S. N. Dixit and V. McKoy, Chem. Phys. Lett. 128, 49 (1986); (d) R. L. Dubs, V. McKoy and S. N. Dixit, J. Chem. Phys. 88, 968 (1988); (e) H. Rudolph and V. McKoy, J. Chem. Phys. 91, 2235 (1989), and references therein to related work by the same group.
33. See, for instance, (a) S. N. Dixit and V. McKoy, J. Chem. Phys. 82, 3546 (1985); (b) S. N. Dixit, D. L. Lynch, and V. McKoy, Phys. Rev. A 32, 1267 (1985); (c) S. N. Dixit and V. McKoy, Chem. Phys. Lett. 128, 49 (1986); (d) R. L. Dubs, V. McKoy and S. N. Dixit, J. Chem. Phys. 88, 968 (1988); (e) H. Rudolph and V. McKoy, J. Chem. Phys. 91, 2235 (1989), and references therein to related work by the same group.
34. See, for instance, (a) S. N. Dixit and V. McKoy, J. Chem. Phys. 82, 3546 (1985); (b) S. N. Dixit, D. L. Lynch, and V. McKoy, Phys. Rev. A 32, 1267 (1985); (c) S. N. Dixit and V. McKoy, Chem. Phys. Lett. 128, 49 (1986); (d) R. L. Dubs, V. McKoy and S. N. Dixit, J. Chem. Phys. 88, 968 (1988); (e) H. Rudolph and V. McKoy, J. Chem. Phys. 91, 2235 (1989), and references therein to related work by the same group.
35. See, for instance, (a) S. N. Dixit and V. McKoy, J. Chem. Phys. 82, 3546 (1985); (b) S. N. Dixit, D. L. Lynch, and V. McKoy, Phys. Rev. A 32, 1267 (1985); (c) S. N. Dixit and V. McKoy, Chem. Phys. Lett. 128, 49 (1986); (d) R. L. Dubs, V. McKoy and S. N. Dixit, J. Chem. Phys. 88, 968 (1988); (e) H. Rudolph and V. McKoy, J. Chem. Phys. 91, 2235 (1989), and references therein to related work by the same group.
36. G. M. Nathanson and G. M. McClelland, J. Chem. Phys. 81, 629 (1984); Chem. Phys. Lett. 114, 441 (1985).
37. G. M. Nathanson and G. M. McClelland, J. Chem. Phys. 81, 629 (1984); Chem. Phys. Lett. 114, 441 (1985).
38. K. L. Reid, S. P. Duxon, and M. Towrie, Chem. Phys. Lett. 228, 351 (1994).
39. Vibrational autoionization in polyatomics is studied in Ch. Jungen and S. T. Pratt, J. Chem. Phys. 106, 9529 (1997).
40. (a) Electrostatic autoionization is studied, for instance, in M. Raoult, H. LeRouzo, G. Raseev, and H. Lefebvre-Brion, J. Phys. B 16, 4601 (1983);
41. (b) Spin-orbit autoionization is studied, for instance, in H. Lefebvre-Brion. A. Giusti-Suzor and G. Raseev, J. Chem. Phys. 83, 1557 (1985);
42. (c) For a review and examples see H. Lefebvre-Brion, in High Resolution Laser Photoionization and Photoelectron Studies, edited by I. Powis, T. Baer and C. Y. Ng (Wiley, New York, 1995), p. 172 and references therein.
43. R. E. Stratmann and R. R. Lucchese, J. Chem. Phys. 101, 95548 (1994), and references therein.
44. K. Kirby, T. Uzer, A. C. Allison, and A. Dalgarno, J. Chem. Phys. 75, 2820 (1981).
45. See, for instance, (a) P. B. Corkum, Phys. Rev. Lett. 71, 1994 (1993); (b) T. Seideman, M. Yu. Ivanov, and P. B. Corkum, Phys. Rev. Lett. 75, 281 (1995); T. Seideman, M. Yu. Ivanov, and P. B. Corkum, Chem. Phys. Lett. 252, 181 (1996); M. Yu. Ivanov, T. Seideman, P. B. Corkum, P. Dietrich, and F. A. Ilkov, Phys. Rev. A 54, 1541 (1996), and references therein.
46. See, for instance, (a) P. B. Corkum, Phys. Rev. Lett. 71, 1994 (1993); (b) T. Seideman, M. Yu. Ivanov, and P. B. Corkum, Phys. Rev. Lett. 75, 281 (1995); T. Seideman, M. Yu. Ivanov, and P. B. Corkum, Chem. Phys. Lett. 252, 181 (1996); M. Yu. Ivanov, T. Seideman, P. B. Corkum, P. Dietrich, and F. A. Ilkov, Phys. Rev. A 54, 1541 (1996), and references therein.
47. See, for instance, (a) P. B. Corkum, Phys. Rev. Lett. 71, 1994 (1993); (b) T. Seideman, M. Yu. Ivanov, and P. B. Corkum, Phys. Rev. Lett. 75, 281 (1995); T. Seideman, M. Yu. Ivanov, and P. B. Corkum, Chem. Phys. Lett. 252, 181 (1996); M. Yu. Ivanov, T. Seideman, P. B. Corkum, P. Dietrich, and F. A. Ilkov, Phys. Rev. A 54, 1541 (1996), and references therein.
48. See, for instance, (a) P. B. Corkum, Phys. Rev. Lett. 71, 1994 (1993); (b) T. Seideman, M. Yu. Ivanov, and P. B. Corkum, Phys. Rev. Lett. 75, 281 (1995); T. Seideman, M. Yu. Ivanov, and P. B. Corkum, Chem. Phys. Lett. 252, 181 (1996); M. Yu. Ivanov, T. Seideman, P. B. Corkum, P. Dietrich, and F. A. Ilkov, Phys. Rev. A 54, 1541 (1996), and references therein.
49. T. Seideman, J. Chem. Phys. 103, 7887 (1995).
50. See, for instance, D. A. Micha and R. D. Piacentini, Phys. Rev. A 25, 204 (1982).
51. R. N. Zare and D. R. Herschbach, Proc. IEEE 51, 173 (1963).
52. A. R. Edmonds, Angular Momentum in Quantum Mechanics, 2nd ed. (Princeton University Press, Princeton, 1960).
53. R. R. Lucchese, G. Raseev and V. McKoy, Phys. Rev. A 25, 2572 (1982).
54. See, for instance, T. Seideman, Chem. Phys. Lett. 235, 279 (1996).
55. Y. Itakawa, Chem. Phys. 28, 461 (1978).
56. D. A. Baugh, V. A. Cho. J. Petteway, T. Garner, and D. Y. Kim, SPIE Proc. V. 1858, 100 (1993); D. A. Baugh, D. Y. Kim, V. A. Cho, L. C. Pipes, J. C. Petteway, and C. D. Fuglesang, Chem. Phys. Lett. 219, 207 (1994).
57. D. A. Baugh, V. A. Cho. J. Petteway, T. Garner, and D. Y. Kim, SPIE Proc. V. 1858, 100 (1993); D. A. Baugh, D. Y. Kim, V. A. Cho, L. C. Pipes, J. C. Petteway, and C. D. Fuglesang, Chem. Phys. Lett. 219, 207 (1994).
58. C. Cornaggia, A. Giusti-Suzor, and Ch. Jungen, J. Chem. Phys. 87, 3934 (1987).
59. M. Rotenberg, R. Bivis, N. Metropolis, and J. K. Wootens, Jr., 3j and 6j Symbols (Technology, Cambridge, MA 1959).
60. Although not directly related to the theme of the present work, it is worth pointing out that time-resolved photofragment angular distributions are expected to provide valuable complementary information with regard to alignment-modifying interactions such as rotation-vibration coupling and electronic nonadiabaticity. While measurement of the electron signal offers technical advantages, the interpretation of photofragment angular distributions is easier since it relies on knowledge of the photofragmentation, rather than the photoionization transition dipole elements and since the fragmentation dynamics can be often made simple and rapid. We note that vibranonal energy flow was recently studied in the time domain using photodissociation as the probe stage, D. Bingemann, M. P. Gorman, A. M. King, and F. F. Crim, J. Chem. Phys. 107, 661 (1997).
61. See, for example, B. Friedrich and D. R. Herschbach, Z. Phys. D 18, 153 (1991); B. Friedrich, D. R. Herschbach, J.-M. Rost, H-G. Rubahn, M. Renger, and M. Verbeek, J. Chem. Soc. Faraday Trans. 89, 1539 (1993); B. Friedrich, A. Slenczka and D. R. Herschbach, Chem. Phys. Lett. 221, 333 (1994): B. Friedrich and D. R. Herschbach, Phys. Rev. Lett. 74, 4623 (1995).
62. See, for example, B. Friedrich and D. R. Herschbach, Z. Phys. D 18, 153 (1991); B. Friedrich, D. R. Herschbach, J.-M. Rost, H-G. Rubahn, M. Renger, and M. Verbeek, J. Chem. Soc. Faraday Trans. 89, 1539 (1993); B. Friedrich, A. Slenczka and D. R. Herschbach, Chem. Phys. Lett. 221, 333 (1994): B. Friedrich and D. R. Herschbach, Phys. Rev. Lett. 74, 4623 (1995).
63. See, for example, B. Friedrich and D. R. Herschbach, Z. Phys. D 18, 153 (1991); B. Friedrich, D. R. Herschbach, J.-M. Rost, H-G. Rubahn, M. Renger, and M. Verbeek, J. Chem. Soc. Faraday Trans. 89, 1539 (1993); B. Friedrich, A. Slenczka and D. R. Herschbach, Chem. Phys. Lett. 221, 333 (1994): B. Friedrich and D. R. Herschbach, Phys. Rev. Lett. 74, 4623 (1995).
64. See, for example, B. Friedrich and D. R. Herschbach, Z. Phys. D 18, 153 (1991); B. Friedrich, D. R. Herschbach, J.-M. Rost, H-G. Rubahn, M. Renger, and M. Verbeek, J. Chem. Soc. Faraday Trans. 89, 1539 (1993); B. Friedrich, A. Slenczka and D. R. Herschbach, Chem. Phys. Lett. 221, 333 (1994): B. Friedrich and D. R. Herschbach, Phys. Rev. Lett. 74, 4623 (1995).