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A comparable hypochromic shift is also observed by the compounds with ortho-nitrophenyl at C-2
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We anticipate that because of the push/pull stabilization of the VHF forms, the DHA(a-e)/VHF(a-e) interconversion leads to an off/on switching of second-order hyperpolarizability (ref. [3e]). Qualitatively, the significant positive solvatochromism is strong indication of an exalted second-order hyperpolarizability in VHF (ref. [18a]).
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6 (stored under argon) has to be used.
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, vol.6
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